Below-cloud rain scavenging of atmospheric aerosols for aerosol deposition models

摘要

Below-cloud aerosol scavenging is generally estimated from field measurements using advanced instruments that measure changes in aerosol distributions with respect to rainfall. In this study, we discuss various scavenging mechanisms and scavenging coefficients from past laboratory and field measurements. Scavenging coefficients derived from field measurements (representing natural aerosols scavenging) are two orders higher than that of theoretical ones for smaller particles (D_p<2 μm). Measured size-resolved scavenging coefficients can be served as a better option to the default scavenging coefficient (e.g. a constant of 10~(-4) s~(-1) for all size of aerosols, as used in the CALPUFF model) for representing below-cloud aerosol scavenging. We propose scavenging correction parameter (C_r) as an exponential function of size-resolved scavenging coefficients, winds and width in the downwind of the source-receptor system. For a wind speed of 3 m s~(-1), C_R decrease with the width in the downwind for particles of diameters D_p<0.1 urn but C_R does not vary much for particles in the accumulation mode (0.1