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首页> 外文期刊>Atmospheric environment >Uncertainties of isoprene emissions in the MEGAN model estimated for a coniferous and broad-leaved mixed forest in Southern China
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Uncertainties of isoprene emissions in the MEGAN model estimated for a coniferous and broad-leaved mixed forest in Southern China

机译:MEGAN模型中估计的中国南方针叶阔叶混交林中异戊二烯排放的不确定性

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摘要

With local observed emission factor and meteorological data, this study constrained the Model of Emissions of Gases and Aerosols from Nature (MEGAN) v2.1 to estimate isoprene emission from the Dinghushan forest during fall 2008 and quantify the uncertainties associated with MEGAN parameters using Monte Carlo approach. Compared with observation-based isoprene emission data originated from a campaign during this period at this site, the local constrained MEGAN tends to reproduce the diurnal variations and magnitude of isoprene emission reasonably well, with correlation coefficient of 0.7 and mean bias of 47.5%. The results also indicate high uncertainties in isoprene emission estimated, with the relative error varied from -89.0-111.0% at the 95% confidence interval. The key uncertainty sources include emission factors, γ_(TLD). photosynthetically active radiation (PAR) and temperature. This implies that accurate input of emission factor, PAR and temperature is a key approach to reduce uncertainties in isoprene emission estimation.
机译:利用当地观察到的排放因子和气象数据,本研究限制了自然气体和气溶胶排放模型(MEGAN)v2.1的估计,以估算2008年秋季鼎湖山森林的异戊二烯排放,并使用蒙特卡洛方法量化了与MEGAN参数相关的不确定性方法。与此期间在该地点开展的一次运动得出的基于观测的异戊二烯排放数据相比,局部受约束的MEGAN趋向于很好地再现异戊二烯排放的昼夜变化和幅度,相关系数为0.7,平均偏差为47.5%。结果还表明估计的异戊二烯排放具有高度不确定性,相对误差在95%置信区间内为-89.0-111.0%。关键的不确定性来源包括排放因子γ_(TLD)。光合有效辐射(PAR)和温度。这意味着准确输入排放因子,PAR和温度是减少异戊二烯排放估算中不确定性的关键方法。

著录项

  • 来源
    《Atmospheric environment》 |2014年第12期|105-110|共6页
  • 作者单位

    School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China;

    School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China;

    Pacific Northwest National Laboratory, Richland, WA 99532, USA;

    State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China;

    State Key Laboratory of Organic Geochemistry, Guangzhou Institute of Geochemistry, Chinese Academy of Science, Guangzhou 510640, China;

    School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China;

    School of Environmental Science and Engineering, Sun Yat-sen University, Guangzhou 510275, China;

    Key Laboratory of Climate-Environment for East Asia, Institute of Atmospheric Physics, Chinese Academy of Sciences, Beijing 100029, China;

  • 收录信息
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    MEGAN; Isoprene emission; Uncertainty; Monte Carlo; Dinghushan; Biogenic VOCs;

    机译:梅根异戊二烯排放;不确定;蒙特卡洛;鼎湖山生物VOC;

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