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Well-width-dependent carrier lifetime in AlGaN/AlGaN quantum wells

机译:AlGaN / AlGaN量子阱中与阱宽度有关的载流子寿命

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A set of Al_(0.35)Ga_(0.65)N/Al_(0.49)Ga_(0.51)N multiple quantum wells (MQWs) with fixed barrier width and well widths varying from 1.65 to 5.0 nm has been grown by metal-organic chemical vapor deposition. Carrier dynamics in the MQWs were studied using time-resolved photoluminescence (PL) spectroscopy and light-induced transient grating (four wave mixing) technique. The authors observed that the lifetime of nonequilibrium carriers (excitons) increases with decreasing well width and interpreted the effect by stronger localization preventing their migration to nonradiative recombination centers. Meanwhile the radiative decay time is also influenced by screening of the built-in electric field, which spatially separates the electrons and holes. It is shown that this effect affects the initial part of PL intensity decay after pulsed excitation. It becomes more pronounced with increase in the initial carrier density but saturates when the carrier density is high enough to completely screen the built-in electric field. The screening effect on PL decay is stronger in wider quantum wells.
机译:通过金属有机化学气相法生长了一组具有固定势垒宽度和阱宽度在1.65至5.0 nm之间变化的Al_(0.35)Ga_(0.65)N / Al_(0.49)Ga_(0.51)N多量子阱(MQW)沉积。使用时间分辨光致发光(PL)光谱和光诱导瞬态光栅(四波混频)技术研究了MQW中的载流子动力学。作者观察到,非平衡载流子(激子)的寿命随着阱宽度的减小而增加,并通过更强的定位来防止这种现象迁移到非辐射重组中心,从而解释了这种效应。同时,辐射衰减时间还受内置电场屏蔽的影响,该内置电场在空间上将电子和空穴分开。结果表明,这种影响会影响脉冲激发后PL强度衰减的初始部分。随着初始载流子密度的增加,它变得更加明显,但是当载流子密度足够高以完全屏蔽内置电场时,它就会饱和。在更宽的量子阱中,对PL衰变的屏蔽作用更强。

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