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Calibrating the single-wall carbon nanotube resonance Raman intensity by high resolution transmission electron microscopy for a spectroscopy-based diameter distribution determination

机译:通过高分辨率透射电子显微镜校准单壁碳纳米管共振拉曼强度,用于基于光谱的直径分布确定

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摘要

We study a single-wall carbon nanotube (SWNT) sample grown by water-assisted chemical vapor deposition with both resonance Raman scattering (RRS) and high resolution transmission electron microscopy. High resolution transmission electron microscopy measurements of 395 SWNTs determined the diameter distribution of the sample, allowing us to calibrate an RRS radial breathing mode (RBM) map obtained with 51 laser excitation energies from 1.26 to 1.73 eV. Thus, we determined the diameter dependence of the RRS RBM cross-section, which in turn allows the determination of the diameter distribution of any SWNT sample by measuring the RBM Raman signal.
机译:我们研究了通过水辅助化学气相沉积与共振拉曼散射(RRS)和高分辨率透射电子显微镜一起生长的单壁碳纳米管(SWNT)样品。 395个SWNT的高分辨率透射电子显微镜测量确定了样品的直径分布,从而使我们能够校准使用51种激光激发能从1.26至1.73 eV获得的RRS径向呼吸模式(RBM)图。因此,我们确定了RRS RBM横截面的直径依赖性,从而可以通过测量RBM拉曼信号来确定任何SWNT样品的直径分布。

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  • 来源
    《Applied Physicsletters》 |2010年第5期|051910.1-051910.3|共3页
  • 作者单位

    Departamento de Fisica, Universidade Federal de Minas Gerais, 30123-970 Belo Horizonte, Brazil;

    rnDepartamento de Fisica, Universidade Federal de Minas Gerais, 30123-970 Belo Horizonte, Brazil;

    ERC Inc/NASA Johnson Space Center, Mail Stop ES-4, P.O. Box 58561, Houston, Texas 77258, USA;

    rnChemistry Division, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA;

    rnNanotube Research Center, National Institute of Advanced Industrial Science and Technology (AIST),Tsukuba, 305-8565, Japan;

    Department of Physics, Tohoku University, Sendai 980-8578, Japan;

    rnDepartment of Physics and Department of Electrical Engineering and Computer Science, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA;

    rnDepartamento de Fisica, Universidade Federal de Minas Gerais, 30123-970 Belo Horizonte, Brazil Divisao de Metrologia de Materials, Instituto Nacional de Metrologia, Normalizacao e Qualidade Industrial (INMETRO), Duque de Caxias, 25250-020 RJ, Brazil;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
  • 原文格式 PDF
  • 正文语种 eng
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  • 入库时间 2022-08-18 03:18:40

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