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Carbon dots decorated vertical SnS_2 nanosheets for efficient photocatalytic oxygen evolution

机译:碳点装饰垂直SnS_2纳米片可有效释放光催化氧气

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摘要

Metal sulfides are highly desirable materials for photocatalytic water splitting because of their appropriate energy bands. However, the poor stability under light illumination in water hinders their wide applications. Here, two-dimensional SnS_2 nanosheets, along with carbon dots of the size around 10 nm, are uniformly grown on fluorine doped tin oxide glasses with a layer of nickel nano-particles. Significantly, strong light absorption and enhanced photocurrent density are achieved after integration of SnS_2 nanosheets with carbon dots. Notably, the rate of oxygen evolution reached up to l.lmmol g~(-1) h~(-1) under simulated sunlight irradiation featuring a good stability.
机译:金属硫化物由于其合适的能带而成为光催化水分解的高度希望的材料。但是,在水中的光照下稳定性差,阻碍了它们的广泛应用。在此,二维SnS_2纳米片以及大小为10 nm左右的碳点在带有镍纳米粒子层的掺氟氧化锡玻璃上均匀生长。重要的是,在将SnS_2纳米片与碳点整合后,实现了强光吸收和增强的光电流密度。值得注意的是,在模拟的阳光照射下,氧气的释放速率达到了1.1mmol g〜(-1)h〜(-1),具有良好的稳定性。

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  • 来源
    《Applied Physics Letters》 |2016年第5期|053905.1-053905.4|共4页
  • 作者单位

    School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, China ,CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

    School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

    CAS Key Laboratory of Nanosystem and Hierarchical Fabrication, National Center for Nanoscience and Technology, Beijing 100190, China ,CAS Center for Excellence in Nanoscience, National Center for Nanoscience and Technology, Beijing 100190, China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
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  • 正文语种 eng
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  • 入库时间 2022-08-18 03:14:46

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