Estimation of 99Mo production rates from natural molybdenum in research reactors

摘要

Molybdenum-99 is one of the most important radionuclides for medical diagnostics. In 2015, the International Atomic Energy Agency organized a round-robin exercise where the participants measured and calculated specific saturation activities achievable for the ⁹⁸Mo(n,γ)⁹⁹Mo reaction. This reaction is of interest as a means to locally, and on a small scale, produce ⁹⁹Mo from natural molybdenum. The current paper summarises a set of experimental results and reviews the methodology for calculating the corresponding saturation activities. Activation by epithermal neutrons and also epithermal neutron self-shielding are found to be of high importance in this case.