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Radiative Decay Engineering 6: Fluorescence on One-Dimensional Photonic Crystals

机译:辐射衰减工程6:一维光子晶体上的荧光

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摘要

During the past decade the interactions of fluorophores with metallic particles and surfaces has become an active area of research. These near-field interactions of fluorophores with surface plasmons have resulted in increased brightness and directional emission. However, using metals provide some disadvantages, like quenching at short fluorophore-metal distances, increased rates of energy dissipation due to lossy metals. These unfavorable effects are not expected in dielectrics. In this paper we describe the interactions of fluorophores with one-dimensional (1D) photonic crystals (PCs), which have alternating layers of dielectrics with dimensions that create a photonic bandgap (PBG). Freely propagating light at the PBG wavelength will be reflected. However, similar with metals, we show that fluorophores within near-field distances of the 1DPC interacts with the structure. Our results demonstrated that these fluorophores can interact with both Internal Modes (IM) and Bloch Surface Waves (BSW) of the 1DPC. For fluorophores on the surface of the 1DPC the emission dominantly occurs through the 1DPC and into the substrate. We refer to these two phenomena together as Bragg Grating-Coupled Emission (BGCE). Here we describe our preliminary results on BGCE. 1DPCs are simple to fabricate and can be handled and reused without damage. We believe BGCE provide opportunities for new formats for fluorescence detection and sensing.
机译:在过去的十年中,荧光团与金属颗粒和表面的相互作用已成为研究的活跃领域。荧光团与表面等离子体激元的这些近场相互作用导致亮度和定向发射增加。但是,使用金属具有一些缺点,例如在较短的荧光团-金属距离处进行淬灭,由于有损金属而导致的能量耗散率增加。在电介质中不会预期这些不利影响。在本文中,我们描述了荧光团与一维(1D)光子晶体(PC)的相互作用,该晶体具有交替的电介质层,其尺寸会产生光子带隙(PBG)。在PBG波长处自由传播的光将被反射。但是,与金属相似,我们表明1DPC的近场距离内的荧光团与结构相互作用。我们的结果表明,这些荧光团可以与1DPC的内部模式(IM)和Bloch表面波(BSW)相互作用。对于1DPC表面上的荧光团,发射主要通过1DPC进入基材。我们将这两种现象统称为布拉格光栅耦合发射(BGCE)。在这里,我们描述了有关BGCE的初步结果。 1DPC易于制造,可以处理和重复使用而不会造成损坏。我们相信BGCE为荧光检测和传感的新格式提供了机会。

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