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Relaxation Oscillations and Ultrafast Emission Pulses in a Disordered Expanding Polariton Condensate

机译:无序膨胀极化子冷凝物中的弛豫振荡和超快发射脉冲

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摘要

Semiconductor microcavities are often influenced by structural imperfections, which can disturb the flow and dynamics of exciton-polariton condensates. Additionally, in exciton-polariton condensates there is a variety of dynamical scenarios and instabilities, owing to the properties of the incoherent excitonic reservoir. We investigate the dynamics of an exciton-polariton condensate which emerges in semiconductor microcavity subject to disorder, which determines its spatial and temporal behaviour. Our experimental data revealed complex burst-like time evolution under non-resonant optical pulsed excitation. The temporal patterns of the condensate emission result from the intrinsic disorder and are driven by properties of the excitonic reservoir, which decay in time much slower with respect to the polariton condensate lifetime. This feature entails a relaxation oscillation in polariton condensate formation, resulting in ultrafast emission pulses of coherent polariton field. The experimental data can be well reproduced by numerical simulations, where the condensate is coupled to the excitonic reservoir described by a set of rate equations. Theory suggests the existence of slow reservoir temporarily emptied by stimulated scattering to the condensate, generating ultrashort pulses of the condensate emission.
机译:半导体微腔通常受结构缺陷的影响,这些结构缺陷会干扰激子-极化子冷凝物的流动和动力学。此外,由于非相干激子储层的性质,激子-极化子冷凝物中存在各种动力学情况和不稳定性。我们研究激子-极化子冷凝物的动力学,这种现象出现在半导体微腔中受到紊乱的影响,这决定了其时空行为。我们的实验数据揭示了在非共振光脉冲激发下复杂的突发状时间演化。凝结水排放的时间模式是由内在的紊乱引起的,并且受激子储层性质的驱动,激子水库的时间衰减相对于极化子凝结水寿命而言要慢得多。此功能在极化子凝聚物中形成弛豫振荡,导致相干极化子场的超快发射脉冲。通过数值模拟可以很好地再现实验数据,其中冷凝物耦合到由一组速率方程描述的激子油藏。理论表明,缓慢的储层的存在是由于受激散射到凝析油中而暂时清空的,从而产生凝析油排放的超短脉冲。

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