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Optical nano-woodpiles: large-area metallic photonic crystals and metamaterials

机译:光学纳米木桩:大面积金属光子晶体和超材料

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摘要

Metallic woodpile photonic crystals and metamaterials operating across the visible spectrum are extremely difficult to construct over large areas, because of the intricate three-dimensional nanostructures and sub-50 nm features demanded. Previous routes use electron-beam lithography or direct laser writing but widespread application is restricted by their expense and low throughput. Scalable approaches including soft lithography, colloidal self-assembly, and interference holography, produce structures limited in feature size, material durability, or geometry. By multiply stacking gold nanowire flexible gratings, we demonstrate a scalable high-fidelity approach for fabricating flexible metallic woodpile photonic crystals, with features down to 10 nm produced in bulk and at low cost. Control of stacking sequence, asymmetry, and orientation elicits great control, with visible-wavelength band-gap reflections exceeding 60%, and with strong induced chirality. Such flexible and stretchable architectures can produce metamaterials with refractive index near zero, and are easily tuned across the IR and visible ranges.
机译:由于需要复杂的三维纳米结构和亚50微米以下的特性,因此在大范围内难以构造在可见光谱范围内工作的金属木桩光子晶体和超材料。先前的路线使用电子束光刻或直接激光写入,但是广泛的应用受到其费用和低产量的限制。包括软光刻,胶体自组装和干涉全息术在内的可扩展方法产生的结构在特征尺寸,材料耐用性或几何形状方面受到限制。通过多次堆叠金纳米线柔性光栅,我们展示了一种可扩展的高保真度方法,用于制造柔性金属木桩光子晶体,具有批量生产且成本低至10 nm的特征。堆叠顺序,不对称性和方向的控制引起了极大的控制,可见光波段的带隙反射超过60%,并且具有很强的手性。这种灵活且可拉伸的体系结构可以产生折射率接近零的超材料,并且可以轻松地在IR和可见范围内进行调整。

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