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Spectral interferometric microscopy reveals absorption by individual optical nanoantennas from extinction phase

机译:光谱干涉显微镜显示消光相中单个光学纳米天线的吸收

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摘要

Optical antennas transform light from freely propagating waves into highly localized excitations that interact strongly with matter. Unlike their radio frequency counterparts, optical antennas are nanoscopic and high frequency, making amplitude and phase measurements challenging and leaving some information hidden. Here we report a novel spectral interferometric microscopy technique to expose the amplitude and phase response of individual optical antennas across an octave of the visible to near-infrared spectrum. Although it is a far-field technique, we show that knowledge of the extinction phase allows quantitative estimation of nanoantenna absorption, which is a near-field quantity. To verify our method we characterize gold ring-disk dimers exhibiting Fano interference. Our results reveal that Fano interference only cancels a bright mode’s scattering, leaving residual extinction dominated by absorption. Spectral interference microscopy has the potential for real-time and single-shot phase and amplitude investigations of isolated quantum and classical antennas with applications across the physical and life sciences.
机译:光学天线将光从自由传播的波转换为高度局限的激发,与物质强烈相互作用。与它们的射频对应物不同,光学天线是纳米和高频的,这使得幅度和相位测量具有挑战性,并且隐藏了一些信息。在这里,我们报告了一种新颖的光谱干涉显微技术,可在可见光到近红外光谱的八度范围内显示单个光学天线的幅度和相位响应。尽管这是一种远场技术,但我们证明了消光阶段的知识允许对纳米天线吸收(这是一个近场量)进行定量估计。为了验证我们的方法,我们对表现出Fano干扰的金环盘二聚体进行了表征。我们的结果表明,法诺干涉仅能消除明亮模式的散射,而剩余的消光则主要由吸收引起。频谱干涉显微镜具有对孤立的量子天线和经典天线进行实时和单次相位和幅度研究的潜力,在物理和生命科学领域都有广泛的应用。

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