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Simultaneous loss of interlayer coherence and long-range magnetism in quasi-two-dimensional PdCrO2

机译:准二维PdCrO2中层间相干性和远距离磁性的同时损失

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摘要

In many layered metals, coherent propagation of electronic excitations is often confined to the highly conducting planes. While strong electron correlations and/or proximity to an ordered phase are believed to be the drivers of this electron confinement, it is still not known what triggers the loss of interlayer coherence in a number of layered systems with strong magnetic fluctuations, such as cuprates. Here, we show that a definitive signature of interlayer coherence in the metallic-layered triangular antiferromagnet PdCrO2 vanishes at the Néel transition temperature. Comparison with the relevant energy scales and with the isostructural non-magnetic PdCoO2 reveals that the interlayer incoherence is driven by the growth of short-range magnetic fluctuations. This establishes a connection between long-range order and interlayer coherence in PdCrO2 and suggests that in many other low-dimensional conductors, incoherent interlayer transport also arises from the strong interaction between the (tunnelling) electrons and fluctuations of some underlying order.
机译:在许多层状金属中,电子激发的相干传播通常局限于高导电平面。尽管强电子相关性和/或接近有序相被认为是这种电子限制的驱动因素,但在许多具有强烈磁波动的层状系统(例如铜酸盐)中,触发层间相干性损失的原因仍然未知。在这里,我们表明,在Néel转变温度下,金属层状三角反铁磁体PdCrO2中层间相干性的明确特征消失了。与相关能级和同构非磁性PdCoO2的比较表明,层间不相干性是由短程磁波动的增长驱动的。这在PdCrO2中的长程有序和层间相干之间建立了联系,并表明在许多其他低维导体中,不相干的层间传输也源于(隧道形)电子之间的强相互作用和某些基本秩序的波动。

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