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Correlated electronic states at domain walls of a Mott-charge-density-wave insulator 1T-TaS2

机译:Mott电荷密度波绝缘体1T-TaS2的畴壁处的相关电子态

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摘要

Domain walls in interacting electronic systems can have distinct localized states, which often govern physical properties and may lead to unprecedented functionalities and novel devices. However, electronic states within domain walls themselves have not been clearly identified and understood for strongly correlated electron systems. Here, we resolve the electronic states localized on domain walls in a Mott-charge-density-wave insulator 1T-TaS2 using scanning tunneling spectroscopy. We establish that the domain wall state decomposes into two nonconducting states located at the center of domain walls and edges of domains. Theoretical calculations reveal their atomistic origin as the local reconstruction of domain walls under the strong influence of electron correlation. Our results introduce a concept for the domain wall electronic property, the walls own internal degrees of freedom, which is potentially related to the controllability of domain wall electronic properties.
机译:交互电子系统中的畴壁可以具有不同的局部状态,这些局部状态通常支配物理属性,并可能导致空前的功能和新颖的设备。但是,对于强相关的电子系统,尚未清楚地识别和理解畴壁内的电子状态。在这里,我们使用扫描隧道光谱法解析位于Mott电荷密度波绝缘体1T-TaS2中的畴壁上的电子状态。我们确定畴壁状态分解为位于畴壁中心和畴边缘的两个非导电状态。理论计算表明,在电子相关性的强烈影响下,它们的原子起源是畴壁的局部重建。我们的结果引入了畴壁电子特性的概念,即壁具有内部自由度,这可能与畴壁电子特性的可控性有关。

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