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Enhanced superconductivity close to a non-magnetic quantum critical point in electron-doped strontium titanate

机译:电子掺杂钛酸锶中接近非磁性量子临界点的增强超导性

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摘要

Studies on quantum critical points (QCP) have focused on magnetic QCPs to date. Remarkable phenomena such as superconductivity due to avoided criticality have been discovered, but we focus here on the non-magnetic counterpart, i.e., the superconductivity of SrTiO3 regarded as being close to a ferroelectric QCP. Here we prepare high-quality Sr1−xLaxTi(16O1−z18Oz)3 single crystals without localisation at low temperatures, which allow us to systematically investigate the La substitution of Sr as an alternative to introducing oxygen vacancies. Analysis of our data based on a theoretical model predicts an appearance of the ferroelectric QCP around 3 × 1018 cm−3. Because of the QCP, the superconducting dome of Sr1−xLaxTiO3 can be raised upwards. Furthermore, remarkable enhancement of Tc (~0.6 K) is achieved by 18O exchange on the Sr1−xLaxTiO3 crystals. These findings provide a new knob for observing intriguing physics around the ferroelectric QCP.
机译:迄今为止,关于量子临界点(QCP)的研究都集中在磁性QCP上。已经发现了显着的现象,例如由于避免了临界而导致的超导性,但是在这里我们集中于非磁性的对应物,即被认为接近铁电QCP的SrTiO3的超导性。在这里,我们制备了高质量的Sr1-xLaxTi( 16 O1-z 18 Oz)3单晶,没有在低温下的局限性,这使我们能够系统地研究La的取代Sr作为引入氧空位的替代方法。基于理论模型对我们的数据进行分析,可以预测铁电QCP的出现在3×10 18 cm -3 附近。由于QCP,Sr1-xLaxTiO3的超导圆顶可以向上升高。此外,通过在Sr1-xLaxTiO3晶体上进行 18 O交换,可显着提高Tc(〜0.6 K)。这些发现为观察铁电QCP周围有趣的物理学提供了新的旋钮。

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