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High-order harmonic generation from the dressed autoionizing states

机译:从修整的自电离态产生高次谐波

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摘要

In high-order harmonic generation, resonant harmonics (RH) are sources of intense, coherent extreme-ultraviolet radiation. However, intensity enhancement of RH only occurs for a single harmonic order, making it challenging to generate short attosecond pulses. Moreover, the mechanism involved behind such RH was circumstantial, because of the lack of direct experimental proofs. Here, we demonstrate the exact quantum paths that electron follows for RH generation using tin, showing that it involves not only the autoionizing state, but also a harmonic generation from dressed-AIS that appears as two coherent satellite harmonics at frequencies ±2Ω from the RH (Ω represents laser frequency). Our observations of harmonic emission from dressed states open the possibilities of generating intense and broadband attosecond pulses, thus contributing to future applications in attosecond science, as well as the perspective of studying the femtosecond and attosecond dynamics of autoionizing states.
机译:在高次谐波的产生中,谐振谐波(RH)是强烈的,相干的极紫外辐射的来源。但是,RH的强度增强仅在单个谐波阶次上发生,这使得生成短的阿秒脉冲具有挑战性。而且,由于缺乏直接的实验证据,这种RH背后的机制是偶然的。在这里,我们演示了电子在使用锡产生RH时遵循的确切量子路径,表明它不仅涉及自电离态,而且还涉及由修整AIS产生的谐波,该谐波出现为两个相干卫星谐波,相对于RH的频率为±2Ω (Ω表示激光频率)。我们对穿戴态谐波发射的观察打开了产生强且宽带的阿秒脉冲的可能性,从而有助于未来在阿秒科学中的应用以及研究自动电离态的飞秒和阿秒动力学的观点。

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