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Tunable Microcavity-Stabilized Quantum Cascade Laser for Mid-IR High-Resolution Spectroscopy and Sensing

机译:用于中红外高分辨率光谱和传感的可调谐微腔稳定量子级联激光器

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摘要

The need for highly performing and stable methods for mid-IR molecular sensing and metrology pushes towards the development of more and more compact and robust systems. Among the innovative solutions aimed at answering the need for stable mid-IR references are crystalline microresonators, which have recently shown excellent capabilities for frequency stabilization and linewidth narrowing of quantum cascade lasers with compact setups. In this work, we report on the first system for mid-IR high-resolution spectroscopy based on a quantum cascade laser locked to a CaF2 microresonator. Electronic locking narrows the laser linewidth by one order of magnitude and guarantees good stability over long timescales, allowing, at the same time, an easy way for finely tuning the laser frequency over the molecular absorption line. Improvements in terms of resolution and frequency stability of the source are demonstrated by direct sub-Doppler recording of a molecular line.
机译:对用于中红外分子传感和计量的高性能和稳定方法的需求推动了越来越紧凑和耐用系统的开发。旨在满足对稳定的中红外参考的需求的创新解决方案之一是晶体微谐振器,该晶体微谐振器最近展示了出色的功能,可通过紧凑的设置实现量子级联激光器的频率稳定和线宽变窄。在这项工作中,我们报告了基于锁定在CaF2微谐振器上的量子级联激光器的第一个用于中红外高分辨率光谱的系统。电子锁定将激光线宽缩小一个数量级,并保证了长时间范围内的良好稳定性,同时允许在分子吸收线上微调激光频率的简便方法。通过分子线的直接亚多普勒记录,证明了信号源的分辨率和频率稳定性方面的改进。

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