首页> 美国卫生研究院文献>Micromachines >AC Electrokinetics of Polarizable Tri-Axial Ellipsoidal Nano-Antennas and Quantum Dot Manipulation
【2h】

AC Electrokinetics of Polarizable Tri-Axial Ellipsoidal Nano-Antennas and Quantum Dot Manipulation

机译:可极化三轴椭圆形纳米天线的交流电动力学和量子点操纵

代理获取
本网站仅为用户提供外文OA文献查询和代理获取服务,本网站没有原文。下单后我们将采用程序或人工为您竭诚获取高质量的原文,但由于OA文献来源多样且变更频繁,仍可能出现获取不到、文献不完整或与标题不符等情况,如果获取不到我们将提供退款服务。请知悉。

摘要

By realizing the advantages of using a tri-axial ellipsoidal nano-antenna (NA) surrounded by a solute for enhancing light emission of near-by dye molecules, we analyze the possibility of controlling and manipulating the location of quantum dots (similar to optical tweezers) placed near NA stagnation points, by means of prevalent AC electric forcing techniques. First, we consider the nonlinear electrokinetic problem of a freely suspended, uncharged, polarized ellipsoidal nanoparticle immersed in a symmetric unbounded electrolyte which is subjected to a uniform AC ambient electric field. Under the assumption of small Peclet and Reynolds numbers, thin Debye layer and ‘weak-field’, we solve the corresponding electrostatic and hydrodynamic problems. Explicit expressions for the induced velocity, pressure, and vorticity fields in the solute are then found in terms of the Lamé functions by solving the non-homogeneous Stokes equation forced by the Coulombic density term. The particular axisymmetric quadrupole-type flow for a conducting sphere is also found as a limiting case. It is finally demonstrated that stable or equilibrium (saddle-like) positions of a single molecule can indeed be achieved near stagnation points, depending on the directions of the electric forcing and the induced hydrodynamic (electroosmotic) and dielectrophoretic dynamical effects. The precise position of a fluorophore next to an ellipsoidal NA, can thus be simply controlled by adjusting the frequency of the ambient AC electric field.
机译:通过认识到使用溶质包围的三轴椭圆形纳米天线(NA)来增强附近染料分子的发光的优势,我们分析了控制和操纵量子点位置的可能性(类似于光学镊子) )通过流行的交流电强制技术放置在NA停滞点附近。首先,我们考虑了一个自由悬浮的,不带电的,极化的椭圆形纳米粒子浸入对​​称的无边界电解质中的非线性动力学问题,该电解质受到均匀的交流环境电场的作用。在小Peclet和雷诺数,薄的德拜层和“弱场”的假设下,我们解决了相应的静电和流体动力学问题。然后,通过求解由库仑密度项强迫的非均匀斯托克斯方程,根据Lamé函数找到溶质中感应速度,压力和涡度场的显式表达式。还发现用于导电球体的特定轴对称四极型流动是极限情况。最终证明,取决于电强迫的方向以及诱导的流体动力学(电渗)和介电泳动力学效应,实际上可以在停滞点附近实现单个分子的稳定或平衡(类似鞍形)的位置。因此,可以通过调节环境AC电场的频率来简单地控制荧光团在椭圆形NA旁边的精确位置。

著录项

相似文献

  • 外文文献
  • 中文文献
  • 专利
代理获取

客服邮箱:kefu@zhangqiaokeyan.com

京公网安备:11010802029741号 ICP备案号:京ICP备15016152号-6 六维联合信息科技 (北京) 有限公司©版权所有
  • 客服微信

  • 服务号