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In situ frequency gating and beam splitting of vacuum- and extreme-ultraviolet pulses

机译:真空和极紫外脉冲的原位频率门控和分束

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摘要

Monochromatization of high-harmonic sources has opened fascinating perspectives regarding time-resolved photoemission from all phases of matter. Such studies have invariably involved the use of spectral filters or spectrally dispersive optical components that are inherently lossy and technically complex. Here we present a new technique for the spectral selection of near-threshold harmonics and their spatial separation from the driving beams without any optical elements. We discover the existence of a narrow phase-matching gate resulting from the combination of the non-collinear generation geometry in an extended medium, atomic resonances and absorption. Our technique offers a filter contrast of up to 104 for the selected harmonics against the adjacent ones and offers multiple temporally synchronized beamlets in a single unified scheme. We demonstrate the selective generation of 133, 80 or 56 nm femtosecond pulses from a 400-nm driver, which is specific to the target gas. These results open new pathways towards phase-sensitive multi-pulse spectroscopy in the vacuum- and extreme-ultraviolet, and frequency-selective output coupling from enhancement cavities.
机译:高次谐波源的单色化为物质各个阶段的时间分辨光发射开辟了有趣的视角。这些研究总是涉及固有地有损且技术复杂的光谱滤光片或光谱色散光学组件的使用。在这里,我们提出了一种新的技术,用于近阈值谐波的频谱选择及其在没有任何光学元件的情况下与驱动光束的空间分离。我们发现由于在扩展的介质中非共线生成几何,原子共振和吸收的结合而导致存在窄相位匹配门。对于选定的谐波,我们的技术针对相邻谐波提供了高达10 4 的滤波器对比度,并在单个统一方案中提供了多个时间同步子束。我们演示了从400 nm驱动器选择性生成133、80或56?nm飞秒脉冲的过程,该脉冲特定于目标气体。这些结果为在真空和极紫外光中进行相敏多脉冲光谱以及增强腔的频率选择性输出耦合开辟了新的途径。

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