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Risk Assessment of Metals in Urban Soils from a Typical Industrial City Suzhou Eastern China

机译:中国东部典型工业城市城市土壤中金属的风险评估

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摘要

Risk of metals in urban soils is less studied, compared to that in other types of soils, hindering accurate assessment of human exposure to metals. In this study, the concentrations of five metals (As, Cd, Cr, Pb, and Hg) were analyzed in 167 surface soil samples collected from Suzhou city and their potential ecological and human health risks were assessed. The mean concentrations of As, Cd, Pb, and Hg except Cr, were higher than the background values in Jiangsu Province. Metal concentrations varied among districts, where sites of high contamination showed a punctate distribution. Principal components and correlation analyses revealed that As, Pb, and Cd could originate from the same sources. The geo-accumulation (Igeo) and potential ecological risk indices (RI) were calculated and the relatively low values of Igeo (<0) and RI (<150) suggested generally low ecological risk. The noncarcinogenic risks of the metals were relatively low for Suzhou residents (i.e., average hazard index or HI: 0.1199 for adults and 0.5935 for children, <1), while the total carcinogenic risks (TCR) of Cr and As were acceptable (TCR in the range of 1.0 × 10−6 to 1.0 × 10−4). Children faced a higher threat than adults. Results of Monte-Carlo simulations were lower than those obtained from models using deterministic parameters. Of all the uncertain parameters, the ingestion rate and body weight were the most sensitive for adults and children, respectively, while As was an important factor for both. The results as well as the factors controlling risks of metals could help better understand the risks of metals in urban soils of industrial cities in China.
机译:与其他类型的土壤相比,对城市土壤中金属风险的研究较少,这妨碍了人们对金属暴露的准确评估。在这项研究中,分析了从苏州市收集的167个表层土壤样品中的五种金属(砷,镉,铬,铅,铅和汞)的浓度,并评估了其潜在的生态和人类健康风险。除Cr外,As,Cd,Pb和Hg的平均浓度高于江苏省的背景值。不同地区之间的金属浓度各不相同,在这些地区高污染的地点呈点状分布。主成分和相关分析表明,As,Pb和Cd可能源自相同的来源。计算了地质累积量(Igeo)和潜在生态风险指数(RI),并且Igeo(<0)和RI(<150)的相对较低值表明总体上生态风险较低。苏州居民的金属非致癌风险相对较低(即平均危害指数或HI:成人为0.1199,儿童为0.5935,<1),而铬和砷的总致癌风险(TCR)是可以接受的( 1.0×10 −6 到1.0×10 −4 的范围)。儿童面对的威胁要比成年人大。蒙特卡洛模拟的结果低于使用确定性参数的模型获得的结果。在所有不确定的参数中,摄入速率和体重分别对成人和儿童最为敏感,而As是两者的重要因素。结果以及控制金属风险的因素有助于更好地了解中国工业城市土壤中金属的风险。

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