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Light scattering studies of irregularly shaped particles.

机译:不规则形状颗粒的光散射研究。

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摘要

We present light scattering studies of irregularly shaped particles which significantly affect the climate. We built and calibrated our apparatus which was able to measure all six independent scattering matrix elements. Our apparatus detects light from 0.32° to 157° simultaneously. We studied all six scattering matrix elements of irregularly shaped Arizona Road Dust which behave differently than those of spheres. We strongly focused on the most important scattering matrix element---the phase function, scattered intensity vs. the scattering angle, which we applied Q-space analysis to. Q-space analysis involves plotting the scattering intensity vs. the magnitude of the scattering wave vector q or qR with R the radius of a particle, on a double logarithmic scale. We measured and studied the phase functions of Al2O3 abrasives; compared the scattering from the abrasives with the scattering of spheres.;To generalize the study, we collected a large amount of experimental and theoretical data from our group and others and applied Q-space analysis. They all displayed a common scattering pattern. The power law exponents showed a quasi-universal functionality with the internal coupling parameter rho'. In situ studies of the soot fractal aggregates produced from a burner were also conducted. A power law exponent -1.85 is seen to imply the aggregates have fractal dimension of Df = 1.85.;The overall work presented shows Q-space analysis uncovers patterns common to all particles: a q-independent forward scattering regime is followed by a Guinier regime, a power law regime, and sometimes an enhanced back scattering regime. The description of the patterns applies to spheres as well, except the power law regime has more than a single power law. These simple patterns give a unified description for all particle shapes. Moreover, the power law exponents have a quasi-universal functionality with rho' for non-fractal aggregates. The absolute value of the exponents start from 4 when rho' is small. As rho' increases, the exponents decrease until the trend levels off at rho' ≥ 10 where the exponents reach a constant 1.75 +/- 0.25. All the non-fractal particles fall on the same trend regardless of the detail of their structure.
机译:我们目前对不规则形状的颗粒进行光散射研究,这些颗粒会严重影响气候。我们构建并校准了能够测量所有六个独立散射矩阵元素的设备。我们的设备可同时检测0.32°至157°的光线。我们研究了形状不规则的亚利桑那州道路扬尘的所有六个散射矩阵元素,其行为与球体不同。我们重点关注最重要的散射矩阵元素-相函数,散射强度与散射角,我们将其应用于Q空间分析。 Q空间分析包括以双对数标度绘制散射强度与散射波矢量q或qR的大小的关系,其中R为粒子的半径。我们测量并研究了Al2O3磨料的相函数;将磨料的散射与球体的散射进行了比较;为了概括研究,我们从小组和其他人那里收集了大量的实验和理论数据,并进行了Q空间分析。它们都显示出共同的散射图案。幂律指数显示出具有内部耦合参数rho'的拟通用函数。还对燃烧器产生的烟灰分形聚集体进行了原位研究。幂律指数为-1.85,表明聚集体的分形维数为Df = 1.85 .;所展示的整体工作表明Q空间分析揭示了所有粒子共有的模式:独立于q的前向散射体制后是Guinier体制,幂律制度,有时是增强的反向散射制度。模式的描述也适用于领域,除了权力法制度不仅仅具有单一的权力法。这些简单的模式为所有粒子形状提供了统一的描述。此外,幂定律指数对于非分形集合体具有rho'的拟通用泛函。当rho'小时,指数的绝对值从4开始。随着rho'的增加,指数将减小,直到趋势稳定在rho'≥10时为止,此时指数达到恒定的1.75 +/- 0.25。无论其结构的细节如何,所有非分形粒子都具有相同的趋势。

著录项

  • 作者

    Heinson, Yuli Wang.;

  • 作者单位

    Kansas State University.;

  • 授予单位 Kansas State University.;
  • 学科 Physics.;Climate change.
  • 学位 Ph.D.
  • 年度 2016
  • 页码 120 p.
  • 总页数 120
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

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