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Methods for coherent lensless imaging and X-ray wavefront measurements.

机译:相干无透镜成像和X射线波前测量的方法。

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摘要

X-ray diffractive imaging is set apart from other high-resolution imaging techniques (e.g. scanning electron or atomic force microscopy) for its high penetration depth, which enables tomographic 3D imaging of thick samples and buried structures. Furthermore, using short x-ray pulses, it enables the capability to take ultrafast snapshots, giving a unique opportunity to probe nanoscale dynamics at femtosecond time scales. In this thesis we present improvements to phase retrieval algorithms, assess their performance through numerical simulations, and develop new methods for both imaging and wavefront measurement.;Building on the original work by Faulkner and Rodenburg, we developed an improved reconstruction algorithm for phase retrieval with transverse translations of the object relative to the illumination beam. Based on gradient-based nonlinear optimization, this algorithm is capable of estimating the object, and at the same time refining the initial knowledge of the incident illumination and the object translations. The advantages of this algorithm over the original iterative transform approach are shown through numerical simulations.;Phase retrieval has already shown substantial success in wavefront sensing at optical wavelengths. Although in principle the algorithms can be used at any wavelength, in practice the focus-diversity mechanism that makes optical phase retrieval robust is not practical to implement for x-rays. In this thesis we also describe the novel application of phase retrieval with transverse translations to the problem of x-ray wavefront sensing. This approach allows the characterization of the complex-valued x-ray field in-situ and at-wavelength and has several practical and algorithmic advantages over conventional focused beam measurement techniques. A few of these advantages include improved robustness through diverse measurements, reconstruction from far-field intensity measurements only, and significant relaxation of experimental requirements over other beam characterization approaches. Furthermore, we show that a one-dimensional version of this technique can be used to characterize an x-ray line focus produced by a cylindrical focusing element. We provide experimental demonstrations of the latter at hard x-ray wavelengths, where we have characterized the beams focused by a kinoform lens and an elliptical mirror. In both experiments the reconstructions exhibited good agreement with independent measurements, and in the latter a small mirror misalignment was inferred from the phase retrieval reconstruction. These experiments pave the way for the application of robust phase retrieval algorithms for in-situ alignment and performance characterization of x-ray optics for nanofocusing. We also present a study on how transverse translations help with the well-known uniqueness problem of one-dimensional phase retrieval.;We also present a novel method for x-ray holography that is capable of reconstructing an image using an off-axis extended reference in a non-iterative computation, greatly generalizing an earlier approach by Podorov et al. The approach, based on the numerical application of derivatives on the field autocorrelation, was developed from first mathematical principles. We conducted a thorough theoretical study to develop technical and intuitive understanding of this technique and derived sufficient separation conditions required for an artifact-free reconstruction. We studied the effects of missing information in the Fourier domain, and of an imperfect reference, and we provide a signal-to-noise ratio comparison with the more traditional approach of Fourier transform holography. We demonstrated this new holographic approach through proof-of-principle optical experiments and later experimentally at soft x-ray wavelengths, where we compared its performance to Fourier transform holography, iterative phase retrieval and state-of-the-art zone-plate x-ray imaging techniques (scanning and full-field). Finally, we present a demonstration of the technique using a single 20 fs pulse from a high-harmonic table-top source. Holography with an extended reference is shown to provide fast, good quality images that are robust to noise and artifacts that arise from missing information due to a beam stop. (Abstract shortened by UMI.)
机译:X射线衍射成像具有高穿透深度,与其他高分辨率成像技术(例如扫描电子或原子力显微镜)不同,可以对厚样品和掩埋结构进行3D层析成像。此外,使用短的X射线脉冲,它可以拍摄超快的快照,从而为在飞秒时间尺度上探测纳米级动力学提供了独特的机会。在本文中,我们提出了相位检索算法的改进,通过数值模拟评估其性能,并开发了用于成像和波前测量的新方法。;在Faulkner和Rodenburg的原始工作的基础上,我们开发了一种改进的相位检索重建算法。物体相对于照明光束的横向平移。该算法基于基于梯度的非线性优化,能够估计物体,同时完善入射照明和物体平移的初始知识。通过数值仿真显示了该算法相对于原始迭代变换方法的优势。相恢复已经显示出在光波长下的波前感测中的巨大成功。尽管原则上该算法可以在任何波长下使用,但实际上,使光学相位恢复更可靠的聚焦分集机制对于X射线而言并不可行。在本文中,我们还描述了具有横向平移的相位检索在X射线波前感测问题中的新型应用。这种方法允许在原位和在波长处表征复值x射线场,并且与常规聚焦光束测量技术相比,具有一些实用和算法优势。这些优点中的一些优点包括通过各种测量来提高鲁棒性,仅从远场强度测量中进行重建以及与其他光束表征方法相比大大放宽了实验要求。此外,我们表明该技术的一维版本可用于表征由圆柱状聚焦元件产生的X射线线聚焦。我们提供了在硬X射线波长下的后者的实验演示,在该演示中,我们表征了由kinoform透镜和椭圆镜聚焦的光束。在两个实验中,重建与独立的测量结果都显示出良好的一致性,在后者中,从相位恢复重建中推断出较小的镜面未对准。这些实验为稳健的相位检索算法的应用铺平了道路,该算法用于纳米聚焦的X射线光学器件的原位对准和性能表征。我们还提出了关于横向平移如何帮助解决一维相位检索的众所周知的唯一性问题的研究;我们还提出了一种X射线全息术的新方法,该方法能够使用离轴扩展参考重建图像在非迭代计算中,极大地推广了Podorov等人的较早方法。该方法基于导数在场自相关上的数值应用,是从第一项数学原理发展而来的。我们进行了深入的理论研究,以发展对该技术的技术性和直观性的理解,并得出了无伪影重建所需的足够分离条件。我们研究了傅立叶域中信息丢失以及参考文献不完善的影响,并与傅立叶变换全息术的更传统方法进行了信噪比比较。我们通过原理证明的光学实验证明了这种新的全息方法,随后在软X射线波长下进行了实验,我们将其性能与傅立叶变换全息术,迭代相位恢复和最新的波带片x-射线成像技术(扫描和全视场)。最后,我们展示了使用高谐波桌面来源的单个20 fs脉冲的技术演示。显示了具有扩展参考的全息图,可以提供快速,高质量的图像,这些图像对于由于波束停止而丢失信息而产生的噪声和伪影具有鲁棒性。 (摘要由UMI缩短。)

著录项

  • 作者

    Guizar Sicairos, Manuel.;

  • 作者单位

    University of Rochester.;

  • 授予单位 University of Rochester.;
  • 学科 Physics Optics.
  • 学位 Ph.D.
  • 年度 2010
  • 页码 282 p.
  • 总页数 282
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

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