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(Invited) Resonant Electroluminescence from Suspended Carbon Nanotube pn-junctions

机译:(邀请)来自悬浮碳纳米管PN-结的共振电致发光

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There are various mechanisms of light emission in carbon nanotubes (CNTs), which give rise to a wide range of spectral characteristics that provide important information regarding the underlying physical processes of photon emission. Here, we report resonant electroluminescence in suspended carbon nanotube pn-junctions generated from dual gate CNT field effect transistor (FET) devices. By applying equal and opposite voltages to the gate electrodes (i.e., V_(g1) = -V_(g2)), we create a pn-junction within the CNT. Under these gating conditions, we observe a sharp resonance in the electroluminescence intensity around zero applied gate voltages, where the depletion region in the p-i-n device has the largest spatial extent. Here, the emission occurs under high electrical power densities around 0.1 MW/cm~2 (or 6μW) and arises from thermal emission at elevated temperatures above 1000K. It is somewhat surprising that this thermal emission intensity is so sensitive to the gating conditions, and we observe a resonant enhancement factor of 1000-fold between V_(g1)=0V and V_(g1)=15V, over a range in which the electrical power dissipated in the nanotube is roughly constant. This resonant behavior is understood on the basis of two phenomena that occur when the depletion region is aligned with the trench across which the nanotube is suspended: 1.) heating is increased in the suspended region because the nanotube is not directly heat sunk to the underlying substrate and 2.) light emission is enhanced in the suspended region due to reduced non-radiative recombination caused by the underlying substrate. Based on the calculated conduction and valence band profiles in the device, we find that the size of the depletion region drops by a factor of 5-1 OX over the range from |V_g|=0V to 15V. We, therefore, conclude that the light emission intensity is significantly dependent on the length of the depletion region in these CNT devices.
机译:碳纳米管(CNT)中存在各种发光机制,其产生广泛的光谱特性,其提供关于光子发射的底层物理过程的重要信息。这里,我们在从双栅极CNT场效应晶体管(FET)器件中产生的悬浮碳纳米管PN-结中报告共振电致发光。通过向栅电极施加相等和相反的电压(即,V_(G1)= -V_(G2)),我们在CNT内创建PN结。在这些门控条件下,我们观察到零施加栅极电压周围的电致发光强度的急剧共振,其中P-I-N装置中的耗尽区域具有最大的空间程度。这里,发射在大约0.1mW / cm〜2(或6μW)的高电功率密度下发生,并且在1000K以上的升高温度下产生热排放。这种热发射强度对门控条件如此敏感有些令人惊讶的是,在电气的范围内,观察V_(G1)= 0V和V_(G1)= 15V之间的共振增强因子为1000倍。在纳米管中消散的功率大致恒定。当耗尽区与悬浮槽悬浮的沟槽对齐时发生的两种现象是基于两种现象来理解的,因为在悬浮区域中加热增加,因为纳米管不是直接沉入下面的沉降由于由下面的基材引起的非辐射重组,悬浮区域中,在悬浮区域中增强了光学发光。基于装置中的计算的导通和价带分布,我们发现耗尽区的尺寸在G_G | = 0V至15V的范围内下降了5-1焦点。因此,我们得出结论,发光强度显着取决于这些CNT器件中的耗尽区的长度。

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