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MEASUREMENTS OF THERMOPHYSICAL PROPERTIES OF URANIA-GADOLINIA PELLETS BY THE LASER FLASH METHOD

机译:激光闪光法测量铀 - 钆颗粒热物理性质

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The most common fuel used in pressurized water reactors is the uranium dioxide (UO_2). However, there are other modern conceptions of nuclear fuels that have advantages over UO_2. Gadolinium is used as a burnable poison which enables compensation of reactivity and the power distribution adjustment in the reactor core. The utilization of (U,Gd)O_2 fuels instead of separate burnable poison rods is considered in pressurized water reactors for the purpose of extended fuel cycles and higher target burnups. The thermal conductivity of the fuel material is one of the most important properties to evaluate their thermal performance under irradiation. Pellets of (U,Gd)O_2 were produced by uniaxial pressing microspheres and powder of UO_2 mixed with 6wt% of Gd_2O_3 powder, as well as pressing microspheres of uranium and gadolinium mixed oxide (U,Gd)O_2, with concentrations of Gd ranging between 2wt% and 10wt%. The purpose of this study was to determine the thermophysical properties of these (U,Gd)O_2 pellets and compare with the thermal conductivity of a pellet produced by pressing microspheres of UO_2, and taken as a reference, to investigate the effect of gadolinium oxide content on the thermal diffusivity and thermal conductivity of the fuel. The pellets thermophysical properties were measured at the LMPT - Laboratorio de Medicao de Propriedades Termofisicas de Combustiveis Nucleares e Materiais of CDTN - Centro de Desenvolvimento da Tecnologia Nuclear, applying the laser flash method. The thermophysical properties, density, specific heat, thermal diffusivity and thermal conductivity are reported. Values of thermal conductivity varying, in function of the gadolinium content, in the range from 5.57 W·m~(-1)·K~(-1) to 7.74 W·m~(-1)·K~(-1), thermal diffusivity from 1.74×10~(-6) m~2·s~(-1) to 2.36×10~(-6) m~2·s~(-1), and specific heat from 279.26 J·kg~(-1)·K~(-1) to 363.99 J·kg~(-1)·K~(-1), were obtained. The results showed that the addition of gadolinium to UO_2 tends to decrease the thermal conductivity and the specific heat of the fuel.
机译:在压水反应堆中使用的最常见的燃料是二氧化铀(UO_2)。然而,有有超过UO_2优势核燃料等现代观念。钆作为可燃性毒物使反应性的补偿,并在反应堆堆芯中的功率分布的调整。 (U,Gd)的利用率O_2燃料代替单独的可燃烧毒物棒在压水反应堆,延长燃料循环和更高的目标燃耗的目的被认为是。燃料材料的热导率是评估照射下它们的热性能的最重要的性质之一。 (U,Gd)的O_2的颗粒用单轴压制的微球体,并用Gd_2O_3粉末的6%重量,以及混合UO_2的粉末生产的压制(U,Gd)的O_2,铀和钆混合氧化物的微球的钆之间的范围内的浓度2%重量和10%重量。本研究的目的是确定的这些热物理性质(U,Gd)的O_2粒料和用按UO_2的微球所产生的沉淀物的热传导率比较,并作为参考,以调查的氧化钆含量的影响在热扩散系数和燃料的热导率。将粒料热物理性质均在LMPT测量 - 的Laboratorio德Medicao德Propriedades Termofisicas德Combustiveis NuclearesËCDTN的,材料 - 炫酷德Desenvolvimento哒TECNOLOGIA核,施加激光闪光法。热物理性质,密度,比热,热扩散系数和热导率被报告。从5.57 W热传导率变的,在钆含量的函数,在该范围的值·米〜(-1)·K〜(-1),以7.74·W·米〜(-1)·K〜(-1)从1.74×10〜(-6)米热扩散〜2·S〜(-1),以2.36×10〜(-6)米〜2·S〜(-1),和比热从279.26·J·公斤〜(-1)·K〜(-1)到363.99·J·公斤〜(-1)·K〜(-1),获得。该结果表明,添加钆到UO_2趋向于降低热导率和燃料的比热。

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