Efficient conversion of CO2 into valuable chemicals has the potential to reduce net CO2 emissions while generate high-energy density fuels and other commodities. However, reduction of CO2 is very challenging because of its chemical inertness and thermodynamic stability, which typically requires aggressive reaction conditions (high temperature and high pressure). Homogeneous catalytic conversion of CO2 can be carried out at mild condition, but its major drawback of the catalyst recycling together with the reactant solubility limitation and product separation prohibits its large scale application. An ideal catalyst for large-scale industrial CO2 hydrogenation would combine the advantages of homogeneous and heterogeneous catalysts.
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机译：有效转化二氧化碳转化为有价值的化学品，有可能降低净二氧化碳排放，同时产生高能量密度燃料和其他商品。然而，由于其化学惰性和热力学稳定性，CO 2的减少非常具有挑战性，这通常需要腐蚀性反应条件（高温和高压）。 CO 2的均匀催化转化可以在温和条件下进行，但其催化剂的主要缺点与反应物溶解度限制和产品分离一起循环加工，禁止其大规模的应用。用于大型工业CO2氢化的理想催化剂将结合均匀和异质催化剂的优点。
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