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High Precision Size Tuning and Stabilization of Single Salt-Water Microdroplets on a Superhydrophobic Surface

机译:超疏水表面上单盐水微量滴度的高精度尺寸调谐和稳定性

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While their spherical geometry is mostly preserved, salt-water microdroplets can be studied in stable experimental conditions when standing on a superhydrophobic surface. Here, we report how the photothermal effect can be used to continuously tune or lock the whispering gallery mode (WGM) spectrum (therefore the size) of salt-water microdroplets on a superhydrophobic surface. The microdroplets are kept in the controlled atmosphere of a humidity chamber. Local heating by an infrared laser focused at the center of the microdroplet causes it to depart from its equilibrium size, shifting the WGM spectrum. This photothermal tuning effect is fully reversible and can be used to tune the microdroplet radius with a precision reaching 1 A by finely controlling the heating laser power. We demonstrate a new spectroscopy method based on this effect, and use it to measure Q-factors of WGM resonances of up to ~10~5. Conversely, focusing the heating laser to the microdroplet rim causes it to experience absorption resonances, leading to a hysteretic behavior when increasing and decreasing the laser power. We show that this behavior can be used to lock the size of a microdroplet and make it function as an optically bistable element. WGM resonances of microdroplets locked in such a way are probed using a tunable laser, showing a locking precision reaching < 0.01 nm over tens of minutes. These results indicate that the challenges in terms of position and wavelength stability inherent to liquid microdroplets surrounded by air can be overcome, and that they provide an easily tunable and lockable alternative to solid optical microcavities.
机译:虽然它们的球形几何形状主要是保留,盐 - 水微滴可以在稳定的实验条件上的超疏水性表面站立时的研究。在这里,我们报告的光热效应如何可以用来连续地调谐或锁定咸水微滴的回音壁模式(WGM)谱(因此大小)上的超疏水性表面。微滴保持在湿度室中的受控气氛。通过红外激光的局部加热聚焦在微滴导致其从它的平衡尺寸离开中心,移位WGM光谱。这种光热调谐效应是完全可逆的,并且可以用于调整用精密通过精细控制加热激光功率达到1所述的微滴半径。我们证明基于这种效应的新的光谱法,并用它来测量高达〜10〜5的WGM共振的Q-因素。相反地​​,加热用激光聚焦到微滴轮缘它会导致经验吸收共振,导致滞后行为增加和减小激光功率时。我们表明,这种行为可以用来锁定一个微滴的大小,使IT部门作为光学双稳态元件。锁定在这样的方式的微滴WGM谐振正在使用的可调谐激光器探测,示出了锁定精度达到<超过几十分钟的0.01纳米。这些结果表明,在位置和固有的被空气包围液体微滴波长稳定性方面的挑战是可以克服的,并且它们提供容易可调且可锁定的替代固体光学微。

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