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Microscopic Theory of the Linear and Nonlinear Terahertz Response of Semiconductors

机译:半导体线性和非线性太赫兹响应的微观理论

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Terahertz (THz) spectroscopy provides a powerfull method to characterize different quasi-particles in optically excited semiconductors (see, e.g., experiments [1, 2]). When the intra-excitonic 1s-to-2p transition is excited with a strong THz pulse, all kinds of nonlinear and extreme nonlinear effects are observed [3, 4] including Rabi flopping, THz high harmonics, and the excitonic dynamical Franz-Keldysh effect. We present a theoretical analysis of the nonlinear THz response from the internal transitions of coherent [3] and incoherent [4] excitons based on our microscopic THz theory [5, 6]. Moreover, the response of unexcited semiconductors to extremely intense THz fields is investigated (see Fig. 1(a)). For field strengths larger than about 3MV/cm, frequency components up to 200 times the excitation frequency V{sub}0=12THz are generated. This extreme nonlinear high-harmonic generation is caused by the nontrivially coupled dynamics of intraband acceleration and nonresonantly excited interband transitions. Even though the THz field is strongly nonresonant with the bandgap, charge carriers are excited due to multi-photon processes and are then accelerated by the THz field.
机译:Terahertz(THz)光谱提供了一种强大的方法,可以在光学激发半导体中表征不同的准粒子(参见,例如,实验[1,2])。当用强THz脉冲激发激发型1S-to-2P转变时,观察到所有类型的非线性和极端非线性效应[3,4],包括Rabi Flopping,THz高谐波和激子动态Franz-Keldysh效果。我们基于我们的微观THz理论对来自连贯[3]和非连贯[4]激子的内部过渡的非线性THz反应的理论分析[5,6]。此外,研究了未开发的半导体对极其强度THz场的响应(参见图1(a))。对于大于约3mV / cm的场强,产生高达200倍的频率分量V {Sub} 0 = 12Thz。这种极端非线性高谐波生成是由IntraBand加速度的非激动耦合动态和非共振激励的间带转换引起的。尽管THz场与带隙强烈非统治,但由于多光子工艺,电荷载流子被激发,然后通过THz场加速。

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