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Optical transitions and nonlinearities in amorphous Si/SiO2 quantum structures

机译:无定形Si / SiO2量子结构中的光学过渡和非线性

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The interband and intersubband transitions in amorphous Si/SiO$- 2$/ multiple quantum well structures, nonlinear effects, and relations between nonlinearity and electron recombination channels have been investigated. Three types of radiative transitions have been observed: subband-to-subband recombination, recombination between subbands of the well and the impurity states in the barrier layers, and the recombination related to impurity states in the barrier layers. A relaxation of excited carriers between the subbands within the conduction and valence bands has been found that allows one to observe hot luminescence caused by higher subbands of the quantum well. The dependencies of the luminescence intensity on the excitation intensity show that the recombination rate is dependent on the concentration of excited carriers. Intersubband absorption has been observed for the first time in undoped amorphous multiple quantum well structures under interband excitation. The transitions take place between the first and second subband of the conduction band involving nonequilibrium electrons excited in the first subband with optical pumping. The dispersive nonlinearity has been investigated in the Fabry-Perot formed by the top interface of the structure and the substrate. The refractive index changes obtained from intensity dependent reflection spectra depend on the excitation intensity in nonlinear manner and can be described by the model of saturating nonlinearity for lower pump intensity. The nonlinear refractive index reveals resonant behavior associated with the subband structure of the QWs.
机译:研究了无定形Si / SiO $ - 2 $ /多量子阱结构,非线性效应和非线性和电子复合通道之间的间带和三通带转换。已经观察到三种类型的辐射转变:子带到子带重组,井子带的重组和阻挡层中的杂质状态,以及与阻挡层中的杂质态相关的重组。已经发现,在传导和价带内的子带之间放松的振荡载体,其允许人们观察由量子阱的更高亚带引起的热发光。发光强度对激发强度的依赖性表明重组率取决于激发载体的浓度。已经在间带式激励下的未掺杂无定形多量子阱结构中首次观察到三通带吸收。在具有光学泵浦的第一子带中激发的导电带的第一和第二子带之间发生转换。已经在结构和基材的顶部界面形成的法布里 - 珀罗中研究了分散非线性。从强度相关的反射光谱获得的折射率变化取决于非线性方式的激发强度,并且可以通过饱和非线性模型来描述用于更低泵强度的模型。非线性折射率揭示了与QWS的子带结构相关的共振行为。

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