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Evaluation of the IMPROVE Equation for Reconstructing Haze from Speciated Aerosol Data

机译:利用特定气溶胶数据重建雾度的IMPROVE方程的评估

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The Interagency Monitoring of Protected Visual Environments (IMPROVE) protocols for reconstructing ambient light extinction from measured aerosol species are the basis for tracking progress under the Regional Haze Rule. The original IMPROVE algorithm, developed in the mid-1990s, is used to estimate light extinction from the contribution of major aerosol species. The equation also includes hygroscopic and light extinction efficiencies specific to each aerosol species. In 2007 the equation was revised to reflect the most current scientific understanding. Recent research suggests the IMPROVE equation is currently under-predicting measured light scattering coefficients, especially after 2011. In addition, comparisons of reconstructed and measured PM_(2.5) mass suggest that mass reconstruction inherent in the IMPROVE equation is also under-predicting measured mass during this same time period. These results indicate that a review of the current IMPROVE algorithms to reconstruct mass and haze is necessary. As part of this review the assumptions in the algorithms will be evaluated to understand the causes of the under-prediction. A summary of provisional recommendations for refinements to the IMPROVE equation and a discussion of important uncertainties to consider in the assumptions will be discussed. Although tentative recommendations of refinements to the IMPROVE equation are presented, final refinements to the IMPROVE equation await future discussions of the results presented here.
机译:用于根据测得的气溶胶物种重建环境光消光的受保护视觉环境机构间监视(IMPROVE)协议,是根据“区域霾霾法则”跟踪进展的基础。原始的IMPROVE算法于1990年代中期开发,用于根据主要气溶胶物种的贡献来估计消光。该方程式还包括特定于每种气溶胶种类的吸湿和消光效率。在2007年,对方程式进行了修改,以反映最新的科学理解。最近的研究表明,IMPROVE方程当前低估了测得的光散射系数,尤其是在2011年之后。此外,对重建和测量的PM_(2.5)质量的比较表明,IMPROVE方程中固有的质量重构在测量过程中也低估了测量的质量。同一时间段。这些结果表明,有必要对当前的IMPROVE算法进行回顾,以重建质量和雾度。作为本次审查的一部分,将对算法中的假设进行评估,以了解预测不足的原因。将讨论改进IMPROVE方程的临时建议摘要,并讨论在假设中要考虑的重要不确定因素。尽管提出了对IMPROVE方程进行细化的初步建议,但对IMPROVE方程进行了最终的细化仍在等待此处讨论结果的进一步讨论。

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