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Decoupling bulk and surface contributions in water-splitting photocatalysts by in situ ultrafast spectroscopy

机译:通过原位超快光谱法分离水分解光催化剂中的体积和表面贡献

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By performing ultrafast emission spectroscopy in an operating, bias-controlled photoelectrochemical cell, we distinguish between bulk (charge transport) and surface (chemical reaction) recombination processes in a nanostructured photocatalyst and correlate its electronic properties directly with its incident-photon-to-current efficiency.
机译:通过在运行中,偏置控制的光电化学电池中执行超快速发射光谱,我们可以区分纳米结构光催化剂中的本体(电荷传输)和表面(化学反应)重组过程,并将其电子性质直接与其入射光子-电流相关联效率。

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