THERMAL NEUTRON CAPTURE CROSS SECTION OF GADOLINIUM BY PILE-OSCILLATION MEASURMENTS IN MINERVE

摘要

Natural gadolinium is used as a burnable poison in most LWR to account for the excess of reactivity of fresh fuels. For an accurate prediction of the cycle length, its nuclear data and especially its neutron capture cross section needs to be known with a high precision. Recent microscopic measurements at Rensselaer Polytechnic Institute (RPI) suggest a 11% smaller value for the thermal capture cross section of ~(157)Gd, compared with most of evaluated nuclear data libraries. To solve this inconsistency, we have analyzed several pile-oscillation experiments, performed in the MINERVE reactor. They consist in the measurement of the reactivity variation involved by the introduction in the reactor of small-samples, containing different mass amounts of natural gadolinium. The analysis of these experiments is done through the exact perturbation theory, using the PIMS calculation tool, in order to link the reactivity effect to the thermal capture cross section. The measurement of reactivity effects is used to deduce the 2200 m.s~(-1) capture cross section of ~(nat)Gd which is (49360 ± 790) b. This result is in good agreement with the JEFF3.1.1 value (48630 b), within 1.6% uncertainty at la, but is strongly inconsistent with the microscopic measurements at RPI which give (44200 ± 500) b.