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Single-shot ultrafast electron diffraction using electrons accelerated by an intense femtosecond laser pulse

机译:使用强飞秒激光脉冲加速的电子进行单次超快电子衍射

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The key issue to realize single-shot ultrafast electron diffraction (UED) is to develop intense short electron-pulse sources. With conventional UED instruments, an electron pulse is generated at a photocathode irradiated by a femtosecond laser pulse and accelerated by an additional external static electric field. The amount of electrons in the pulse is limited because the electron pulse expands during its flight by space-charge forces in the pulse. There are two ways considerable to avoid the space charge effect; those are reduction of electrons in the pulse and acceleration to relativistic energy by RF accelerators. However, for the former large amount of pulses are necessary to obtain a UED image, which is not available to observe irreversible phenomena, and for the latter the energy is too high for conventional transmission electron microscopy (TEM). Furthermore, for the mid-energy range of around 100keV to 1MeV, corresponding to the energies of conventional TEM, there is no satisfactory method for generating femtosecond electron pulses. In this paper, we have demonstrated femtosecond pulse compression of a laser-accelerated electron beam with energy of around 350keV.[1] The electron pulses are generated by irradiating a tightly focused terawatt femtosecond laser pulse on a solid target; then, the pulses are compressed by using an achromatic bending magnet system. These femtosecond electron pulses have a sufficient intensity to take a single-shot diffraction pattern.[1, 2]
机译:实现单次超快电子衍射(UED)的关键问题是开发强的短电子脉冲源。使用常规的UED仪器,在由飞秒激光脉冲辐照的光电阴极上会产生电子脉冲,并在附加的外部静电电场的作用下加速电子脉冲。脉冲中的电子数量受到限制,因为电子脉冲在其飞行过程中会由于脉冲中的空间电荷力而膨胀。有两种方法可以有效避免空间电荷效应:这些是脉冲中电子的减少以及通过RF加速器加速到相对论能量。但是,对于前者,需要大量脉冲才能获得UED图像,而UED图像不可用于观察不可逆现象,而对于后者,能量对于常规的透射电子显微镜(TEM)而言太高。此外,对于大约100keV到1MeV的中能范围(对应于传统TEM的能量),没有令人满意的产生飞秒电子脉冲的方法。在本文中,我们演示了能量约为350keV的激光加速电子束的飞秒脉冲压缩。[1]电子脉冲是通过将紧密聚焦的太瓦飞秒激光脉冲照射在固体靶上产生的;然后,使用消色差弯曲磁铁系统压缩脉冲。这些飞秒电子脉冲具有足够的强度,可以拍摄单次衍射图。[1,2]

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