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Picosecond nonlinear spectroscopy of quantum-size PbTe films

机译:量子级PbTe薄膜的皮秒非线性光谱

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Abstract: We propose new and promising technique for studying quantum- size structures. We tested this technique based on optical two-photon excitation and probing of renormalized electron spectrum in our investigation of monocrystalline PbTe films. We revealed sharp dependence of spectral position of two- photon resonances versus film thickness L $EQ 6, 18, and 30 nm. Our theoretical model explained this result by taking into account Pb Te band structure, electron-electron and electron-phonon interactions, and redistribution of charge carriers due to inter- and intraband processes. Estimation T$-2$/ $GREQ 300 fs for decay time of interband polarization was obtained.!26
机译:摘要:我们提出了一种研究量子尺寸结构的新技术。我们在单晶PbTe薄膜的研究中基于光学双光子激发和重归一化电子光谱的探测测试了该技术。我们揭示了双光子共振的光谱位置与膜厚度L $ EQ 6、18和30 nm的强烈相关性。我们的理论模型通过考虑Pb Te的能带结构,电子-电子和电子-声子的相互作用以及由于带间和带内过程而造成的电荷载流子的重新分布来解释这一结果。获得带内极化衰减时间的估计T $ -2 $ / $ GREQ 300 fs!26

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