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CATALYST FOR CARBONYLATION OF DIMETHYL ETHER TO PRODUCE METHYL ACETATE, PREPARATION METHOD THEREFOR, AND USE THEREOF
CATALYST FOR CARBONYLATION OF DIMETHYL ETHER TO PRODUCE METHYL ACETATE, PREPARATION METHOD THEREFOR, AND USE THEREOF
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机译:二甲醚羰基化催化剂制备乙酸甲酯,其制备方法及其用途
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摘要
Disclosed are a catalyst for the carbonylation of dimethyl ether to produce methyl acetate, a preparation method therefor, and the use thereof. The catalyst contains a modified H-MOR molecular sieve, wherein the modified H-MOR molecular sieve is prepared by means of the exchange of an H-MOR molecular sieve with a pyridinium salt. Methyl acetate is produced by passing dimethyl ether and a raw material gas containing carbon monoxide through a reactor charged with an acidic molecular sieve catalyst which selectively regulates active sites, and performing a reaction under the conditions of a reaction temperature of 150-280°C, a reaction pressure of 0.5-25.0 MPa, and a space velocity of dimethyl ether of 0.2-4 h -1.
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