The present invention is directed to a self-emulsifiable isocyanate- terminated prepolymer, having an average NCO functionality of from 2.0 to 3.5, which is prepared from: (a) a polyisocyanate mainly composed of at least one of aliphatic polyisocyanates, alicyclic polyisocyanates, and aromatic polyisocyanates, (b-1) a hydrophilic surfactant having at least one active hydrogen group capable of reacting with an isocyanate group, and (b-2) an aliphatic compound of 8 or more carbons, and/or a fatty acid ester in which the total of the carbons of a starting fatty acid and a starting hydroxyl-group-having compound is 8 or more, the aliphatic compound and the fatty acid ester having at least one active hydrogen group capable of reacting with the isocyanate group.
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