A method and system are provided for controlling SNCR performance in a fossil fuel boiler. A performance goal for the boiler and data on current boiler performance is obtained. A determination is made as to whether the performance goal is satisfied by the current boiler performance. When the performance goal is not satisfied, the generally closest operating region in which the performance goal would be satisfied is identified. The operating region is associated with desired operating parameters of one or more devices affecting SNCR performance. One or more control moves are determined using the desired operating parameters of the one or more devices for directing the boiler to the operating region. The one or more control moves are communicated to the one or more devices.
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