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Water borne transport of high level nuclear waste in very deep borehole disposal of high level nuclear waste

机译:在高深度核废料的深井钻井处置中水载运输高放废物

摘要

The purpose of this report is to examine the feasibility of the very deep borehole experiment and to determine if it is a reasonable method of storing high level nuclear waste for an extended period of time. The objective of this thesis is to determine the escape mechanisms of radionuclides and to determine if naturally occurring salinity gradients could counteract this phenomenon. Because of the large dependence on the water density, the relationship between water density and the salinity was measured and agreed with the literature values with a less than 1% difference. The resultant relationship between the density and salinity is a linear relationship with the molality, and dependent upon the number of ions of the dissolved salt (e.g. CaCl₂ contains 3 and NaCl has 2). From the data, it was calculated that within a borehole with a host rock porosity of 10-⁵ Darcy, it would take approximately 10⁵ years for the radionuclides to escape. As the rock porosity decreases, the escape time scale increases, and the escape fraction decreases exponentially. Due to the conservative nature of the calculations, the actual escape timescale would be closer to 106 years and dominated by 1-129 in a reducing atmosphere. The expected borehole salinity values can offset the buoyancy effect due to a 50°C temperature increase.
机译:本报告的目的是研究深井钻孔实验的可行性,并确定是否是将高水平核废料长时间存储的合理方法。本文的目的是确定放射性核素的逸出机理,并确定自然发生的盐度梯度是否可以抵消这种现象。由于对水密度的依赖性很大,因此测量了水密度与盐度之间的关系,并与文献值相符,相差不到1%。密度和盐度之间的最终关系与摩尔浓度呈线性关系,并取决于溶解盐的离子数(例如,CaCl 2含有3个,NaCl具有2个)。根据这些数据,可以计算出,在一个孔隙度为10-⁵Darcy的井眼中,放射性核素逸出大约需要10⁵年。随着岩石孔隙度的降低,逸出时间尺度增加,逸出分数呈指数下降。由于计算的保守性,实际的逃逸时间尺度将接近106年,并在还原性大气中以1-129为主。预期的井眼盐度值可以抵消由于温度升高50°C而产生的浮力影响。

著录项

  • 作者

    Cabeche Dion Tunick;

  • 作者单位
  • 年度 2011
  • 总页数
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类

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