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Quantifying gas emissions from the 'Millennium Eruption' of Paektu volcano, Democratic Peoples Republic of Korea/China

机译:量化朝鲜民主主义人民共和国/中国白头山火山“千年火山喷发”的气体排放量

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摘要

Paektu volcano (Changbaishan) is a rhyolitic caldera that straddles the border between the Democratic People’s Republic of Korea and China. Its most recent large eruption was the Millennium Eruption (ME; 23 km3 dense rock equivalent) circa 946 CE, which resulted in the release of copious magmatic volatiles (H2O, CO2, sulfur, and halogens). Accurate quantification of volatile yield and composition is critical in assessing volcanogenic climate impacts but is challenging, particularly for events before the satellite era. We use a geochemical technique to quantify volatile composition and upper bounds to yields for the ME by examining trends in incompatible trace and volatile element concentrations in crystal-hosted melt inclusions. We estimate that the ME could have emitted as much as 45 Tg of S to the atmosphere. This is greater than the quantity of S released by the 1815 eruption of Tambora, which contributed to the “year without a summer.” Our maximum gas yield estimates place the ME among the strongest emitters of climate-forcing gases in the Common Era. However, ice cores from Greenland record only a relatively weak sulfate signal attributed to the ME. We suggest that other factors came into play in minimizing the glaciochemical signature. This paradoxical case in which high S emissions do not result in a strong glacial sulfate signal may present a way forward in building more generalized models for interpreting which volcanic eruptions have produced large climate impacts.
机译:Paektu火山(长白山)是流纹火山口,横跨朝鲜民主主义人民共和国与中国之间的边界。它最近的一次大喷发是大约在公元946年的千年喷发(ME; 23 km3的致密岩石当量),导致大量岩浆挥发物(H2O,CO2,硫和卤素)释放出来。准确定量挥发物的产量和组成对于评估火山爆发的气候影响至关重要,但具有挑战性,特别是对于卫星时代之前的事件。我们使用地球化学技术通过检查晶体承载的熔体夹杂物中不相容的痕量和挥发性元素浓度趋势来量化ME的挥发性成分和上限。我们估计,ME可能向大气排放了多达45 Tg的S。这比1815年坦波拉火山爆发释放的S量要大,后者促成“没有夏天的一年”。我们的最大天然气产量估算值将ME列为“共同时期”中最强的强迫性气候排放国。然而,格陵兰岛的冰芯仅记录了归因于ME的相对较弱的硫酸盐信号。我们建议其他因素在最小化冰川化学特征中起作用。这种高硫排放不会导致强烈的冰河硫酸盐信号的自相矛盾的情况,可能会为建立更通用的模型以解释哪些火山喷发对气候造成重大影响提供了前进的方向。

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