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Long-lived atmospheric trace gases measurements in flask samples from three stations in India

机译:印度三个站点的烧瓶样品中的长寿命大气痕量气体测量

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摘要

With the rapid growth in population and economic development, emissions ofgreenhouse gases (GHGs) from the Indian subcontinent have sharply increasedduring recent decades. However, evaluation of regional fluxes of GHGs andcharacterization of their spatial and temporal variations by atmosphericinversions remain uncertain due to a sparse regional atmospheric observationnetwork. As a result of an Indo-French collaboration, three new atmosphericstations were established in India at Hanle (HLE), Pondicherry (PON) andPort Blair (PBL), with the objective of monitoring the atmosphericconcentrations of GHGs and other trace gases. Here we present the results ofthe measurements of CO, CH, NO, SF, CO, and Hfrom regular flask sampling at these three stations over the period2007–2011. For each species, annual means, seasonal cycles and gradientsbetween stations were calculated and related to variations in naturalGHG fluxes, anthropogenic emissions, and monsoon circulations.Covariances between species at the synoptic scale were analyzed toinvestigate the likely source(s) of emissions. The flask measurements ofvarious trace gases at the three stations have the potential to constrain theinversions of fluxes over southern and northeastern India. However, thisnetwork of ground stations needs further extension to other parts of Indiato better constrain the GHG budgets at regional and continental scales.
机译:随着人口和经济发展的迅速增长,近几十年来,印度次大陆的温室气体(GHG)排放量急剧增加。然而,由于稀疏的区域大气观测网络,对温室气体区域通量的评估以及通过大气反演表征其空间和时间变化的特征仍然不确定。印法合作的结果是,在印度的汉勒(HLE),本地治里(PON)和布莱尔港(PBL)建立了三个新的大气站,目的是监测温室气体和其他微量气体的大气浓度。在这里,我们介绍了2007年至2011年这三个站点的常规烧瓶采样中CO,CH,NO,SF,CO和H的测量结果。对于每个物种,计算了站之间的年均值,季节周期和梯度,并与自然GHG通量,人为排放和季风环流有关。分析了天气尺度上物种之间的协方差,以调查可能的排放源。在这三个站进行的烧瓶中各种痕量气体的测量可能会限制印度南部和东北部通量的反转。但是,这个地面站网络需要进一步扩展到印度其他地区,以更好地限制区域和大陆规模的温室气体预算。

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