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Atomic layer etching of graphene for full graphene device fabrication

机译:石墨烯原子层蚀刻用于全石墨烯器件制造

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摘要

The possibility of fabricating a full graphene device was investigated by utilizing atomic layer etching (ALET) technology. By using O2 ALET which functions by oxygen radical adsorption followed by the removal of the oxygen chemisorbed on carbon, the removal of exactly one graphene layer per ALET cycle was detected through the increase of the transmittance by 2.3 after one ALET cycle and by the decrease of the G peak in the Raman spectra. The Raman spectra also showed an increase of the D peak after ALET, indicating the formation of physical damage on the graphene surface layer. This damage was mostly recovered by hydrogen annealing at 1000 °C after ALET. Full graphene field effect transistors (source, drain: 3 layer, channel: 1, 2, 3 layer) were fabricated by reducing the channel layers using ALET, followed by annealing, and the electrical characteristics of the devices showed the possibility of fabricating fully functional graphene devices composed of an all graphene source/drain and graphene channel by utilizing ALET.
机译:利用原子层刻蚀(ALET)技术研究了制造完整石墨烯器件的可能性。通过使用氧自由基吸附起作用的O2 ALET,然后去除碳上的氧化学吸附,通过一个ALET循环后透射率增加2.3%和拉曼光谱中G峰的降低,检测到每个ALET循环中正好去除一个石墨烯层。拉曼光谱也显示ALET后D峰增加,表明石墨烯表层上形成了物理损伤。ALET后,这种损伤主要通过1000 °C的氢气退火来恢复。采用ALET还原沟道层,然后进行退火,制备了全石墨烯场效应晶体管(源极、漏极:3层,沟道:1、2、3层),器件的电学特性表明,利用ALET制备由全石墨烯源极/漏极和石墨烯沟道组成的全功能石墨烯器件成为可能。

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