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Twist Angle Tuning of Moire? Exciton Polaritons in van der Waals Heterostructures

机译:莫尔纹的扭转角度调整?范德华异质结构中的激子极化激元

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摘要

Twisted atomically thin semiconductors are characterized by moire?? excitons. Their optical signatures and selection rules are well understood. However, their hybridization with photons in the strong coupling regime for heterostructures integrated in an optical cavity has not been the focus of research yet. Here, we combine an excitonic density matrix formalism with a Hopfield approach to provide microscopic insights into moire?? exciton polaritons. In particular, we show that exciton-light coupling, polariton energy, and even the number of polariton branches can be controlled via the twist angle. We find that these new hybrid light-exciton states become delocalized relative to the constituent excitons due to the mixing with light and higher-energy excitons. The system can be interpreted as a natural quantum metamaterial with a periodicity that can be engineered via the twist angle. Our study presents a significant advance in microscopic understanding and control of moire?? exciton polaritons in twisted atomically thin semiconductors.
机译:扭曲原子薄半导体的特征是摩尔纹??激子。它们的光学特征和选择规则是众所周知的。然而,它们在光腔中集成的异质结构的强耦合机制中与光子的杂化尚未成为研究的重点。在这里,我们将激子密度矩阵形式与霍普菲尔德方法相结合,以提供对摩尔纹的微观见解??激子极化激元。特别是,我们表明激子-光耦合、极化激元能量,甚至极化激元分支的数量都可以通过扭转角来控制。我们发现,由于与光和高能激子的混合,这些新的混合光激子态相对于组成激子变得离域。该系统可以解释为一种天然的量子超材料,其周期性可以通过扭转角进行设计。我们的研究在微观理解和控制云纹方面取得了重大进展??扭曲原子薄半导体中的激子极化激元。

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