Mode of Atmospheric Deposition in Forests Demonstrates Notable Differences in Initial Radiocesium Behavior

摘要

The March 2011 Fukushima Dai-ichi Nuclear Power Plant accident in Japan released S20 PBq of radionuclides compared to a total release of 5300 PBq from the Chornobyl Nuclear Power Plant accident. Both nuclear accidents resulted in deposition of radiocesium throughout the northern hemisphere, and a plethora of studies have been performed regarding radiocesium (~(137)Cs) behavior. However, few studies have assessed the impact of precipitation on ~(137)Cs deposition in forests. Wide-scale environmental measurements from 2011 and 2016 were used to determine the differences in ~(137)Cs deposition because of precipitation following the Fukushima accident. In areas where wet deposition processes were dominant, dense forests generally had lower ambient dose rates and levels of contamination on forest floors than other stands with fewer stems per hectare in 2011. Similar tendencies were not observed in areas that were primarily subject to dry deposition nor were any trends observed in 2016. ~(137)Cs was retained in dense forest canopies for an extended period regardless of the deposition mode. Additionally, it was found that the initial retention of radionuclides by forest canopies is in general higher for areas with predominantly dry deposition. Incorporation of radiocesium into wood tissues was the same for both wet and dry deposition.