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首页> 外文期刊>Journal of environmental radioactivity >Use of STAX data in global-scale simulation of 133Xe atmospheric background
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Use of STAX data in global-scale simulation of 133Xe atmospheric background

机译:STAX数据在133Xe大气背景的全球尺度模拟中的应用

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A global-scale simulation of the 133Xe atmospheric background is automated at the French National Data Center (NDC) for the purpose of categorizing the radionuclide measurements of the Comprehensive Nuclear-Test-Ban Treaty (CTBT) International Monitoring System (IMS). These simulations take into account 133Xe releases from all known major industrial emitters in the world, compiled from the literature and described as constant values. Emission data measured directly at the stack of the Institute for Radio Elements (IRE), a medical isotope production facility located in Fleurus (Belgium), were implemented in the simulations with a time resolution of 15 minutes. This work discusses the contribution of real (measured) emissions to the prediction of the 133Xe atmospheric background at IMS noble gas stations and at a location near Paris, for which IMS-like 133Xe mea-surements were available. For the purpose of this study, simulations initiated with the IRE measured emissions were run in parallel to those with the a priori emissions used to date. The benefits of including actual emissions in the simulations were found as a function of the distance between the station and the source of the release. At the closest stations, i.e., near Paris (France) and at Schauinsland, Freiburg (Germany), respectively 250 and 400 km from Fleurus, the simulated activity concentrations differed by a factor greater than 2 more than one third of the time, and by a factor of more than 5 about 10 of the time. No significant or detectable differences were found beyond 1500-2000 km. Furthermore, at the Paris station, the timing of the measured peaks was better repro-duced with the actual emission data. However, not all peak amplitudes were correctly reproduced even though the real emissions were used, highlighting the remaining uncertainties, primarily in the meteorological data and transport modeling.
机译:法国国家数据中心(NDC)对133Xe大气背景进行了全球规模的模拟,目的是对《全面禁止核试验条约》(全面禁试条约)国际监测系统(IMS)的放射性核素测量值进行分类。这些模拟考虑了世界上所有已知主要工业排放源的133Xe释放,这些释放源自文献并描述为常数值。在位于Fleurus(比利时)的医用同位素生产设施无线电元件研究所(IRE)的烟囱中直接测量的发射数据在模拟中实现,时间分辨率为15分钟。这项工作讨论了实际(测量的)排放对IMS惰性加油站和巴黎附近地点的133Xe大气背景预测的贡献,这些地点可以使用类似IMS的133Xe测量结果。出于本研究的目的,使用IRE测量的排放启动的模拟与迄今为止使用的先验排放的模拟并行运行。在模拟中包括实际排放的好处被发现是站和排放源之间距离的函数。在最近的车站,即,在巴黎(法国)附近和弗莱堡(德国)的绍因斯兰,分别距离弗勒鲁斯250公里和400公里,模拟的活动浓度在超过三分之一的时间内相差大于2倍,在大约10%的时间内相差超过5倍。在1500-2000公里之外没有发现显着或可检测到的差异。此外,在巴黎站,测得的峰值时间与实际排放数据可以更好地再现。然而,即使使用了实际排放量,也未正确再现了所有峰值振幅,这突出了仍然存在的不确定性,主要是在气象数据和传输模型中。

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