Investigating Wetland and Nonwetland Soil Methane Emissions and Sinks Across the Contiguous United States Using a Land Surface Model

摘要

We estimated the distribution of CH(4)emissions and sinks from wetlands (including freshwater and coastal wetlands) and nonwetland (including wet and dry soils) with a newly developed vertically resolved soil CH(4)model, integrated into a global land surface model (ISAM). We calibrated and tested this integrated model with CH(4)observations at test sites in the Contiguous United States (CONUS). ISAM is applied across the CONUS to estimate CH(4)emissions and sinks given both recent past observed climate and wetland extent, and future climate and wetland extent driven by two scenarios, RCP4.5 and RCP8.5. Estimated net CH(4)emissions for the 2000s are 13.8 TgCH(4) yr(-1), mostly from wetland soils. Estimated net emissions under RCP4.5 and RCP8.5 are 30% and 64% higher, respectively, in the 2090s than in the 2000s due to (1) higher temperature and seasonal wetland extent (driven by higher precipitation in the climate scenarios), which increase modeled methanogenic activity more than methanotrophic activity in soils and (2) altered transport in the soil column and exchange with the atmosphere by modeled transport processes (diffusion, ebullition, and aerenchyma transport). Nonwetland soils emit CH4(1.4 TgCH(4) yr(-1)) in some areas and take up CH4(-2.9 TgCH(4) yr(-1)) in other areas, resulting in a net estimated sink for the 2000s; the net nonwetland soil sink increases by 15% and 46% by the 2090s under RCP4.5 and RCP8.5, respectively, mainly due to drier soil conditions, which enhances methanotrophic activity and oxidation of CH(4)diffused into soil from a future atmosphere with higher CH(4)concentration.