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首页> 外文期刊>Journal of Geophysical Research, D. Atmospheres: JGR >Sensitivity of Modeled Soil NOx Emissions to Soil Moisture
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Sensitivity of Modeled Soil NOx Emissions to Soil Moisture

机译:Sensitivity of Modeled Soil NOx Emissions to Soil Moisture

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Abstract As emissions of nitrogen oxides (NOx) from fossil fuel combustion decrease, the relative contribution of NOx emissions from managed and unmanaged soils (SNOx) is increasing. Modeling SNOx presents a challenge as it requires proper characterization of emission dynamics in response to environmental conditions. SNOx is often represented using the Berkeley Dalhousie Soil NOx Parameterization (BDSNP), which relies upon static relationships between soil moisture and SNOx for arid and non‐arid lands. However, soil chamber and atmospheric studies have shown that emission characteristics are more dynamic, with peak emissions often occurring at higher soil moisture content. Here, to better capture observational studies, we update BDSNP by creating a dynamic SNOx response to soil moisture based on a normalized soil moisture index. We compare the standard and updated parameterizations over the contiguous United States (U.S.) for 2011–2020 using input soil moisture data from ERA5‐Land, MERRA‐2 and NLDAS2‐Mosaic and evaluate SNOx across these different input drivers as well as between the standard and updated parameterizations. The standard parametrization exhibits strong sensitivity to different input soil moisture products, with annual U.S. SNOx differences of up to 0.28 Tg N yr−1. In contrast, the updated parameterization provides a robust representation of SNOx with reduced sensitivity to input soil moisture product with differences of at most 0.03 Tg N yr−1. The updated parameterization simulates a broad increase in SNOx in non‐arid regions, including much of the Eastern U.S., indicating that this region may be more sensitive to climatically‐driven SNOx as anthropogenic NOx emissions continue to decline.
机译:摘要随着排放的氮氧化物(NOx)减少化石燃料燃烧的氮氧化物排放量的相对贡献托管和非托管土壤(SNOx)正在增加。因为它需要建模SNOx提出了挑战适当的发射动力学的特征应对环境条件。经常使用伯克利戴尔豪斯表示土壤氮参数化(BDSNP)在静态土壤水分之间的关系和SNOx干旱和非干旱的土地。土壤室和大气研究显示排放特性更有活力,峰值通常发生在更高的排放到大气中土壤含水量。观察性研究,我们更新BDSNP创建一个动态SNOx应对土壤水分基于归一化土壤湿度指数。比较标准和更新在连续的参数化州(美国)2011 - 2020年使用输入土壤从ERA5水分数据量的土地,一2在这些NLDAS2马赛克和评估SNOx不同的输入驱动程序以及之间的标准和更新参数化。标准参数化展示出强大对不同的输入土壤水分的敏感性的产品,每年美国SNOx差异0.28 Tg N年−1。参数化提供了一个健壮的表示敏感性降低的SNOx输入土壤水分最多的产品差异0.03 Tg N年−1。模拟一个广泛SNOx增加非干旱东部地区,包括大部分的美国,表明这个地区可能更敏感地理气候上驱动SNOx人为氮氧化物排放继续下降。

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