Robust Rare‐Earth‐Containing Superhydrophobic Coatings for Strong Protection of Magnesium and Aluminum Alloys

Liu Lei; Lei Jinglei; Li Lingjie; Zhang Jie; Shang Bo; He Jianxin; Li Nianbing; Pan Fusheng

摘要

Abstract > The robust rare‐earth‐containing superhydrophobic coatings are fabricated by a simple and scalable method, which includes spraying the lanthanum hydroxide sol onto metallic substrates (AZ61 Mg and 2024 Al) and then modifying the surfaces with stearic acid. The as‐prepared coatings on AZ61 Mg and 2024 Al have identical morphology and composition. Both are composed of fiber‐like La(OH) <sub>3</sub> nanowires that cross‐link and form a network structure, which are pivotal for inducing surface superhydrophobicity with water contact angles (WCAs) as high as ≈157°. The superhydrophobic coatings demonstrate remarkable corrosion resistance as well as high chemical and mechanical stabilities. The theoretical simulation based on molecular mechanics suggests that the high stabilities mainly arise from the strong bonding between La <sub>2</sub> O <sub>3</sub> and stearic acid molecules. The fabrication approach proposed here is hopeful to extend for large‐scale preparation of robust superhydrophobic metallic materials widely applied. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 通过简单且可伸缩的方法制造了鲁棒稀土的超疏水涂层，其包括将氢氧化镧溶胶喷涂到金属底物（AZ61mg和2024 Al）上，然后用硬脂酸改变表面。 AZ61mg和2024 A1上的AS制备的涂层具有相同的形态和组成。两者都是由纤维状的la（oh）组成 <sub> 3 </ sub> 纳米线，其交联并形成网络结构，该网络结构是用水接触角（WCAS）诱导表面超细侵蚀性高达≈157°的枢转。超疏水涂层表现出显着的耐腐蚀性以及高化学和机械稳定性。基于分子力学的理论模拟表明，高稳定性主要出现在洛杉矶之间的强粘合 <sub> 2 </ sub> O. <sub> 3 </ sub> 和硬脂酸分子。这里提出的制造方法希望延伸用于广泛应用于稳健的超疏水金属材料的大规模制备。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第16期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Lei&option=202" target="_blank" rel="nofollow">Liu Lei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lei Jinglei&option=202" target="_blank" rel="nofollow">Lei Jinglei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Lingjie&option=202" target="_blank" rel="nofollow">Li Lingjie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Jie&option=202" target="_blank" rel="nofollow">Zhang Jie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shang Bo&option=202" target="_blank" rel="nofollow">Shang Bo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Jianxin&option=202" target="_blank" rel="nofollow">He Jianxin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Nianbing&option=202" target="_blank" rel="nofollow">Li Nianbing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pan Fusheng&option=202" target="_blank" rel="nofollow">Pan Fusheng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringChongqing UniversityChongqing 400044 China;</p> <p>School of Chemistry and Chemical EngineeringSouthwest UniversityChongqing 400715 China;</p> <p>School of Materials Science and EngineeringChongqing UniversityChongqing 400044 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=corrosion resistance&option=203" rel="nofollow">corrosion resistance;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molecular mechanics&option=203" rel="nofollow">molecular mechanics;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=rare earth&option=203" rel="nofollow">rare earth;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=stability&option=203" rel="nofollow">stability;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=superhydrophobic coatings&option=203" rel="nofollow">superhydrophobic coatings;</a> </p> <div class="translation"> 机译：耐腐蚀性;分子力学;稀土;稳定性;超疏水涂料; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_transactions-nonferrous-metals-society-china_thesis/0201223186160.html">含有金属黏结相的热喷涂WC涂层在盐雾中的腐蚀行为</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王丽君&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">王丽君,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=邱培现&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">邱培现,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘艳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">刘艳,</a> <a href="/journal-foreign-8190/" target="_blank" rel="nofollow" class="tuijian_authcolor">中国有色金属学报（英文版） .</a> <span>2013</span><span>,第009期</span> </span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-cn_chinese-journal-nonferrous-metals-english_thesis/0201259213449.html">含有金属黏结相的热喷涂WC涂层在盐雾中的腐蚀行为</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王丽君&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">王丽君,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=邱培现&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">邱培现,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=刘艳&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">刘艳,</a> <a href="/journal-foreign-17995/" target="_blank" rel="nofollow" class="tuijian_authcolor">中国有色金属学报：英文版 .</a> <span>2013</span><span>,第009期</span> </span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022435757.html">Superhydrophobicity: Robust Rare‐Earth‐Containing Superhydrophobic Coatings for Strong Protection of Magnesium and Aluminum Alloys (Adv. 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