Tunable Colloidal Crystalline Patterns on Flat and Periodically Micropatterned Surfaces as Antireflective Layers and Printable–Erasable Substrates

Song Ji Eun; Park Jong Seong; Lee Beu; Pyun Seung Beom; Lee Jieun; Kim Min Gyu; Han Yilong; Cho Eun Chul

摘要

Abstract >2D nonclose‐packed colloidal crystal patterns have received considerable attention in various fields, but it remains a challenge to fabricate patterns and manipulate their geometries regardless of substrate types and structures. Herein, a simple approach is developed for producing nonclose‐packed hydrogel colloidal crystalline patterns on flat and periodically micropatterned substrates by exposing close‐packed colloidal crystal monolayers to salt aqueous solutions. The patterns are achievable on flat surfaces like silicon, glass, graphene, poly(ethylene terephthalate), and poly(dimethyl siloxane) surfaces. Hydrogel colloidal spheres can deform into disk‐like or hemispherical particles on different material substrates. The colloid geometries and dimensions in the patterns are tunable by varying the salt type or concentration. The tunable colloidal crystalline patterns can form on periodically micropatterned substrates, resulting in novel hierarchical crystalline structures. The modification of the method is effective to easily fabricate nonclose‐packed hybrid colloidal crystal patterns where plasmonic nanoparticles are selectively assembled on the hydrogel particle surfaces. These patterned substrates modulate colors, reduce reflectivity of visible to near‐infrared light, and enhance transmittance. The nonclose‐packed colloidal patterns are useful as antireflection coating layers to enhance the solar thermoelectricity efficiencies of flat and micropatterned substrates. The optical tunability of colloidal crystal patterns enables developing colloid crystal‐based printable and erasable substrates. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> <P> 2D无卷曲包装的胶体晶体图案在各个领域得到了相当大的关注，而是仍然是制造图案的挑战，并且无论衬底类型和结构如何，操纵它们的几何形状。在此，通过将紧密填充的胶体晶体单层暴露于盐水溶液，开发了一种简单的方法，用于在平坦和周期性的微型底物上产生扁平和周期性的微型底物晶体。在硅，玻璃，石墨烯，聚（乙二醇酯）和聚（二甲基硅氧烷）表面等平坦表面上可实现该图案。水凝胶胶体球可以使不同材料基材上的盘状或半球形颗粒变形。通过改变盐类型或浓度来调谐图案中的胶体几何形状和尺寸。可调谐胶体晶体图案可以在周期性的微图案上形成，导致新颖的分层晶体结构。该方法的改性可有效地易于制造非卷积填充的混合胶体晶体图案，其中等离子体纳米粒子在水凝胶颗粒表面上选择性地组装。这些图案化基板调制颜色，减少可见的近红外光的反射率，并增强透射率。非卷积填充的胶体图案可用作抗反射涂层，以增强扁平和微图案的基板的太阳能热电效率。胶体晶体图案的光学可调性使得能够显影基于胶体晶体的可印刷和可擦除基材。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第11期</span><b style="margin: 0 2px;">|</b><span>共13页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Ji Eun&option=202" target="_blank" rel="nofollow">Song Ji Eun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Park Jong Seong&option=202" target="_blank" rel="nofollow">Park Jong Seong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Beu&option=202" target="_blank" rel="nofollow">Lee Beu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pyun Seung Beom&option=202" target="_blank" rel="nofollow">Pyun Seung Beom;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lee Jieun&option=202" target="_blank" rel="nofollow">Lee Jieun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Kim Min Gyu&option=202" target="_blank" rel="nofollow">Kim Min Gyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Han Yilong&option=202" target="_blank" rel="nofollow">Han Yilong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cho Eun Chul&option=202" target="_blank" rel="nofollow">Cho Eun Chul;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> <p>Department of PhysicsHong Kong University of Science and TechnologyClear Water Bay Hong Kong China;</p> <p>Department of Chemical EngineeringHanyang UniversitySeoul 04763 South Korea;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=geometrically tunable colloidal patterns&option=203" rel="nofollow">geometrically tunable colloidal patterns;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hierarchical colloidal crystal&option=203" rel="nofollow">hierarchical colloidal crystal;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hybrid colloidal crystal&option=203" rel="nofollow">hybrid colloidal crystal;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=light harvesting&option=203" rel="nofollow">light harvesting;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nonclose‐packed colloidal crystal patterns&option=203" rel="nofollow">nonclose‐packed colloidal crystal patterns;</a> </p> <div class="translation"> 机译：几何可调谐胶体图案;分层胶体晶体;混合胶体晶体;光收获;无卷发包装的胶体晶体图案; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> 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