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Quantum interference control of an isolated resonance lifetime in the weak-field limit

机译:弱场限制下的孤立谐振寿命的量子干涉控制

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摘要

Resonance states play an important role in a large variety of physical and chemical processes. Thus, controlling the resonance behavior, and particularly a key property like the resonance lifetime, opens up the possibility of controlling those resonance mediated processes. While such a resonance control is possible by applying strong-field approaches, the development of flexible weak-field control schemes that do not alter significantly the system dynamics still remains a challenge. In this work, one such control scheme within the weak-field regime is proposed for the first time in order to modify the lifetime of an isolated resonance state. The basis of the scheme suggested is quantum interference between two pathways induced by laser fields, that pump wave packet amplitude to the target resonance under control. The simulations reported here show that the scheme allows for both enhancement and quenching of the resonance survival lifetime, being particularly flexible to achieve large lifetime enhancements. Control effects on the resonance lifetime take place only while the pulse is operating. In addition, the conditions required to generate the two interfering quantum pathways are found to be rather easy to meet for general systems, which makes the experimental implementation straightforward and implies the wide applicability of the control scheme.
机译:共振态在多种物理和化学过程中起着重要作用。因此,控制共振行为,特别是诸如共振寿命之类的关键特性,开启了控制那些共振介导过程的可能性。尽管通过应用强磁场方法可以实现这种共振控制,但是开发不会显着改变系统动力学的灵活的弱磁场控制方案仍然是一个挑战。在这项工作中,首次提出了一种在弱场范围内的控制方案,以修改隔离共振状态的寿命。所建议的方案的基础是由激光场引起的两个路径之间的量子干涉,该干涉将波包振幅泵浦到受控的目标共振。此处报道的仿真结果表明,该方案既可以提高共振寿命,也可以淬灭共振寿命,特别灵活,可以实现较大的寿命延长。对谐振寿命的控制影响仅在脉冲运行时发生。另外,发现产生两条干扰量子路径所需的条件对于一般系统而言相当容易满足,这使得实验实现简单明了并且暗示了控制方案的广泛适用性。

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