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On the possibility of electric transport mediated by long living intrinsic localized solectron modes

机译:关于长寿命本征局部电子模式介导的电传输的可能性

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We consider a polaron Hamiltonian in which not only the lattice and the electron-lattice interactions, but also the electron hopping term is affected by anharmonicity. We find that the one-electron ground states of this system are localized in a wide range of the parameter space. Furthermore, low energy excited states, generated either by additional momenta in the lattice sites or by appropriate initial electron conditions, lead to states constituted by a localized electron density and an associated lattice distortion, which move together through the system, at subsonic or supersonic velocities. Thus we investigate here the localized states above the ground state which correspond to moving electrons. We show that besides the stationary localized electron states (proper polaron states) there exist moving localized solectron states which can be easily excited. The evolution of these localized states suggests their potential as new carriers for fast electric charge transport.
机译:我们考虑一个极化子哈密顿量,其中不仅晶格和电子-晶格相互作用,而且电子跳跃项也受非谐性的影响。我们发现,该系统的单电子基态位于较大的参数空间范围内。此外,由晶格位点中的附加动量或适当的初始电子条件产生的低能激发态会导致由局部电子密度和相关的晶格畸变构成的状态,它们以亚音速或超音速的速度一起移动通过系统。因此,我们在这里研究基态以上与移动电子相对应的局部状态。我们表明,除了静止的局部电子态(适当的极化子态)之外,还存在移动的局部电子态,可以很容易地激发它们。这些局部状态的演变表明它们有潜力作为快速电荷传输的新载体。

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