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APPLICATION OF RELAXED EDDY ACCUMULATION TECHNIQUE TO QUANTIFY Hg~0 FLUXES OVER MODIFIED SOIL SURFACES

机译:松弛涡流累积技术在改性土壤表面Hg〜0通量量化中的应用

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摘要

Fluxes of mercury from a waste repository and from an agricultural field amended with sewage sludge were measured. The measurements were performed by utilising a Relaxed Eddy Accumulation (REA) system synchronously coupled to automated mercury cold vapour atomic fluorescence analysers (CVAFA). The waste repository was severely contaminated and fluxes of between 0.16 μg m~(-2) h~(-1) and 29 μg m~(-2) h~(-1) could be measured. Fluxes at the slightly contaminated agricultural field measured between 8 ng m~(-2) h~(-1) and 1.9 μg m~(-2) h~(-1). The results showed that the REA-CVAFA system could be used for measurements above both severely-and slightly contaminated soils. The measurements at the chlor-alkali plant showed that temperature was the most important parameter controlling the release of mercury at this site. At the agricultural field, the measurements indicated that both solar radiation and temperature may have influenced the emissions. Most of the mercury added to the field was lost to the atmosphere during the summer season.
机译:测量了来自废物储存库和经污水污泥修正的农田的汞通量。通过使用松弛涡流累积(REA)系统与自动汞冷蒸气原子荧光分析仪(CVAFA)同步耦合进行测量。废物库受到严重污染,可以测量的通量在0.16μgm〜(-2)h〜(-1)和29μgm〜(-2)h〜(-1)之间。在8 ng m〜(-2)h〜(-1)和1.9μgm〜(-2)h〜(-1)之间的轻微污染农田的通量。结果表明,REA-CVAFA系统可用于在重度和轻度污染土壤上的测量。在氯碱工厂进行的测量表明,温度是控制该地点汞释放的最重要参数。在农业领域,测量结果表明太阳辐射和温度都可能影响排放。夏季,大部分添加到田间的汞都流失到大气中。

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