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首页> 外文期刊>The Science of the Total Environment >The impact of seasonal varied human activity on characteristics and sources of heavy metals in metropolitan road dusts
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The impact of seasonal varied human activity on characteristics and sources of heavy metals in metropolitan road dusts

机译:季节变化的人类活动对都市道路扬尘中重金属的特征和来源的影响

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Due to significant human activity, road dust is becoming contaminated by heavy metals in many cities. To comprehensively investigate the variation of contamination level and sources of heavy metals in road dust, 10 heavy metals in road dust samples from Beijing, China, in both summer and winter, were evaluated by spatial analysis using geographic information system (GIS) mapping technology and the positive matrix factorization (PMF) Model. Although the concentrations of some heavy metals between summer and winter had similarities, the differences of others and spatial distributions of heavy metals between summer and winter were considerable. The mean concentrations of As, Cd, Cr, Cu, and Fe were lower in winter, while those of Hg, Mn, Ni, Pb, and Zn were higher. According to the values of the Pollution Index (PI) and Nemerow Integrated Pollution Index (NIPI), there were no obvious differences between summer and winter, but the range between different sites in winter was nearly twice that of summer. Based on the PMF model, four sources of heavy metals in the dust samples were identified. Although the types of sources were consistent, the relative contributions of each source differed between summer and winter. Non-exhaust vehicle emissions was the most important source in summer (34.47 wt%), while fuel combustion contributed the largest proportion to the total heavy metals in winter (32.40 wt%). The impact of each source also showed spatial variation different trends in summer and winter. With the alteration of seasons, intensity of human activities also changed, such as the number of tourists, energy needs for building temperature regulation, construction, and the amount of pesticides and fertilizer. That might be the reason for the variation of heavy metal concentrations and relative contribution of their sources between summer and winter.
机译:由于人类的大量活动,许多城市的道路灰尘都被重金属污染。为了全面调查道路尘埃的污染水平和重金属来源的变化,使用地理信息系统(GIS)进行空间分析,评估了来自中国北京的夏季和冬季道路尘埃样品中的10种重金属,并正矩阵分解(PMF)模型。尽管夏季和冬季之间某些重金属的浓度具有相似性,但其他一些之间的差异以及夏季和冬季之间重金属的空间分布是相当大的。冬季,砷,镉,铬,铜和铁的平均浓度较低,而汞,锰,镍,铅和锌的平均浓度较高。根据污染指数(PI)和尼梅罗综合污染指数(NIPI)的值,夏季和冬季之间没有明显差异,但冬季不同站点之间的范围几乎是夏季的两倍。基于PMF模型,确定了粉尘样品中的四种重金属来源。尽管来源类型是一致的,但是每个来源的相对贡献在夏季和冬季之间都不同。夏季,非废气排放是最重要的排放源(34.47%wt%),而燃料燃烧占冬季重金属总量的最大比例(32.40%wt%)。在夏季和冬季,每种来源的影响还显示出空间变化的不同趋势。随着季节的变化,人类活动的强度也发生了变化,例如游客人数,建筑温度调节,建筑的能源需求以及农药和化肥的用量。这可能是夏季和冬季之间重金属浓度及其来源相对变化的原因。

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