Magnetic order on a frustrated spin-1/2 Heisenberg antiferromagnet on the Union Jack lattice

摘要

We use the coupled cluster method (CCM) to study the zero-temperature phase diagram of a two-dimensional frustrated spin-half antiferromagnet, the so-called Union Jack model. It is defined on a square lattice such that all nearest-neighbor pairs are connected by bonds with a strength J_1 > 0, but only half the next-nearest-neighbor pairs are connected by bonds with a strength J_2= kJ_1 >0. The bonds are arranged such that on the 2×2 unit cell they form the pattern of the Union Jack flag. Alternating sites on the square lattice are thus four-connected and eight-connected. We find strong evidence for a first phase transition between a Neel antiferromagnetic phase and a canted ferrimagnetic phase at a critical coupling k_(c_1) =0.66 ±0.02. The transition is an interesting one, at which the energy and its first derivative seem continuous, thus providing a typical scenario of a second-order transition (just as in the classical case for the model), although a weakly first-order transition cannot be excluded. By contrast, the average on-site magnetization approaches a nonzero value M_(c_1) =0.195 ± 0.005 on both sides of the transition, which is more typical of a first-order transition. The slope, dM/dk, of the order parameter curve as a function of the coupling strength k, also appears to be continuous, or very nearly so, at the critical point k_(c_1) , thereby providing further evidence of the subtle nature of the transition between the Neel and canted phases. Our CCM calculations provide strong evidence that the canted ferrimagnetic phase becomes unstable at large values of k, and hence we have also used the CCM with a model collinear semistripe-ordered ferrimagnetic state in which alternating rows (and columns) are ferro-magnetically and antiferromagnetically ordered, and in which the spins connected by J_2 bonds are antiparallel to one another. We find tentative evidence, based on the relative energies of the two states, for a second zero-temperature phase transition between the canted and semistripe-ordered ferrimagnetic states at a large value of the coupling parameter around k_(c_2) ≈ 125 ± 5. This prediction, however, is based on an extrapolation of the CCM results for the canted state into regimes where the solutions have already become unstable and the CCM equations based on the canted state at any level of approximation beyond the lowest have no solutions. Our prediction for k_(c_2) is hence less reliable than that for k_(c_1) . Nevertheless, if this second transition at k_(c_1) does exist, our results clearly indicate it to be of first-order type.